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From metal–organic frameworks to single/dual-atom and cluster metal catalysts for energy applications

机译：从金属有机框架到单/双原子和簇金属催化剂的能量应用

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摘要

Single/dual-atom and cluster metal catalysts, with much higher atom-utilization efficiency, remarkable performance, good recyclability and unique properties, have emerged as a new frontier in energy-related catalysis. In recent years, metal-organic frameworks (MOFs) have demonstrated great potential for the targeted creation of single/dual-atom and cluster catalysts, featuring the distinctive advantages of high metal loadings, porous structures and tailorable catalytic sites. In this review, we discuss the key roles and the critical issues of single/dual-atom and cluster catalysts, and the great opportunities furnished by MOFs for the construction strategy. The accessible characterization techniques for single/dual-atom and cluster catalysts will be showcased. Furthermore, we highlight recent advances in the construction and energy applications of MOF-based single/dual-atom and cluster catalysts by taking advantage of structural features of MOFs. Current issues, promising ideas and future prospects for MOF-based single/dual-atom and cluster catalysts are given.
机译：单/双原子和簇金属催化剂，具有更高的原子利用效率，显着性能，良好的可回收性和独特的性质，它被成为能源相关催化的新前沿。近年来，金属 - 有机框架（MOF）已经表现出靶向创造单/双原子和簇催化剂的巨大潜力，具有高金属载荷，多孔结构和可定制的催化位点的独特优势。在这篇综述中，我们讨论了单/双原子和聚类催化剂的关键作用和关键问题，以及由MOF为施工策略提供的巨大机会。将展示单/双原子和簇催化剂的可访问表征技术。此外，我们通过利用MOF的结构特征来突出基于MOF基单/双原子和簇催化剂的近期建筑和能量应用的进展。给出了当前的问题，给出了基于MOF的单/双原子和簇催化剂的承诺想法和未来前景。

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  • 来源
    《Energy & environmental science》 |2020年第6期|1658-1693|共36页
  • 作者

    Hou Chun-Chao; Wang Hao-Fan; Li Caixia; Xu Qiang;

  • 作者单位

    AIST Kyoto Univ Chem Energy Mat Open Innovat Lab ChEM OIL Natl Inst Adv Ind Sci & Technol AIST Sakyo Ku Kyoto 6068501 Japan;

    AIST Kyoto Univ Chem Energy Mat Open Innovat Lab ChEM OIL Natl Inst Adv Ind Sci & Technol AIST Sakyo Ku Kyoto 6068501 Japan;

    AIST Kyoto Univ Chem Energy Mat Open Innovat Lab ChEM OIL Natl Inst Adv Ind Sci & Technol AIST Sakyo Ku Kyoto 6068501 Japan;

    AIST Kyoto Univ Chem Energy Mat Open Innovat Lab ChEM OIL Natl Inst Adv Ind Sci & Technol AIST Sakyo Ku Kyoto 6068501 Japan|Natl Inst Adv Ind Sci & Technol Res Inst Electrochem Energy Ikeda Osaka 5638577 Japan|Yangzhou Univ Sch Chem & Chem Engn Yangzhou 225009 Jiangsu Peoples R China;

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