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Perspective of microporous metal-organic frameworks for CO_2 capture and separation

机译：用于CO_2捕获和分离的微孔金属有机框架的观点

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摘要

It is emergent to reduce carbon dioxide emissions from fossil fuel combustion and thereby limit climate destabilization. In order to achieve the industrial scenario of CCS, there is a need for the discovery of better solid CO_2 adsorbents that realize great improvement of selective capacity and stability to moisture as well as significant reductions in energy requirements and costs. In this review, we provide an overview of the current status of the emerging microporous metal-organic frameworks (MOFs) for the storage and separation of carbon dioxide. We summarize the main factors for CO_2 capture performance of MOF materials under different working conditions, in comparison with those for zeolite materials. At the same time, we analyze the relationship among porous structures, pore/window sizes, capacity, selectivity and enthalpy of porous MOFs for CCS, which will give us clues for the design and synthesis of MOF materials as CO_2 adsorbents.
机译：出现减少化石燃料燃烧产生的二氧化碳排放并由此限制气候不稳定的新兴方法。为了实现CCS的工业应用场景，需要发现更好的固体CO_2吸附剂，该吸附剂可实现对水分的选择性容量和稳定性的极大提高，以及能源需求和成本的显着降低。在本文中，我们概述了新兴的用于存储和分离二氧化碳的微孔金属有机框架（MOF）的现状。我们总结了与沸石材料相比，在不同工作条件下MOF材料的CO_2捕集性能的主要因素。同时，我们分析了多孔MOFs对CCS的多孔结构，孔/窗口尺寸，容量，选择性和焓之间的关系，这将为设计和合成作为CO_2吸附剂的MOF材料提供线索。

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  • 来源
    《Energy & environmental science》 |2014年第9期|2868-2899|共32页
  • 作者

    Zhangjing Zhang; Zi-Zhu Yao; Shengchang Xiang; Banglin Chen;

  • 作者单位

    Fujian Provincial Key Laboratory of Polymer Materials, College of Materials Science and Engineering, Fujian Normal University, Fuzhou, Fujian 350007, China;

    Fujian Provincial Key Laboratory of Polymer Materials, College of Materials Science and Engineering, Fujian Normal University, Fuzhou, Fujian 350007, China;

    Fujian Provincial Key Laboratory of Polymer Materials, College of Materials Science and Engineering, Fujian Normal University, Fuzhou, Fujian 350007, China,College of Life and Environmental Sciences, Minzu University of China, Beijing 100081, China;

    Department of Chemistry, University of Texas at San Antonio, One UTSA Circle, San Antonio, Texas 78249-0698, USA;

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