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Gaseous chemical compounds in indoor and outdoor air of 602 houses throughout Japan in winter and summer

机译:冬季和夏季,全日本602户室内外空气中的气态化合物

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摘要

A nationwide survey of indoor air quality in Japan was conducted using four types of diffusive samplers. Gaseous chemical compounds such as carbonyls, volatile organic compounds (VOC), acid gases, basic gases, and ozone were measured in indoor and outdoor air of 602 houses throughout Japan in winter and summer. Four kinds of diffusive samplers were used in this study: DSD-BPE/DNPH packed with 2,4-dinitrophenyl hydrazine and trans-1,2-bis(2-pyridyl)ethylene coated silica for ozone and carbonyls; VOC-SD packed with Carboxen 564 particles for volatile organic compounds; DSD-TEA packed with trietha-nolamine impregnated silica for acid gases; and DSD-NH_3 packed with phosphoric acid impregnated silica for basic gases. These samplers are small and lightweight and do not require a power source, hence, it was possible to obtain a large number of air samples via mail from throughout Japan. Almost all compounds in indoor air were present at higher levels in summer than in winter. In particular, formaldehyde, toluene, and ammonia were strongly dependent on temperature, and their levels increased with temperature. The nitrogen dioxide concentration in indoor air particularly increased only during winter and was well correlated with the formic acid concentration (correlation coefficient=0.959). Ozone concentrations in indoor air were extremely low compared with the outdoor concentrations. Ozone flowing from outdoor air may be decomposed quickly by chemical compounds in indoor air; therefore, it is suggested that the indoor/outdoor ratio of ozone represents the ventilation of the indoor environment.
机译:日本使用四种类型的扩散采样器对日本的室内空气质量进行了全国范围的调查。在冬季和夏季,在日本全国602户房屋的室内和室外空气中测量了气态化学化合物,如羰基化合物,挥发性有机化合物(VOC),酸性气体,碱性气体和臭氧。本研究中使用了四种扩散采样器:DSD-BPE / DNPH装有2,4-二硝基苯基肼和反式1,2-双(2-吡啶基)乙烯包覆的二氧化硅,用于臭氧和羰基化合物;装有Carboxen 564颗粒的VOC-SD,用于挥发性有机化合物; DSD-TEA填充了三乙胺醇胺浸渍的二氧化硅,用于酸性气体; DSD-NH_3装有磷酸浸渍的二氧化硅,可用于碱性气体。这些采样器体积小,重量轻,不需要电源,因此可以通过邮件从日本各地获取大量空气采样。夏季,室内空气中几乎所有化合物的含量均高于冬季。特别地,甲醛,甲苯和氨强烈依赖于温度,并且它们的含量随温度增加。室内空气中的二氧化氮浓度尤其仅在冬季增加,并且与甲酸浓度高度相关(相关系数= 0.959)。与室外浓度相比,室内空气中的臭氧浓度极低。室外空气中的臭氧可能会被室内空气中的化合物迅速分解;因此,建议臭氧的室内/室外比代表室内环境的通风。

著录项

  • 来源
    《Environmental research》 |2015年第2期|364-372|共9页
  • 作者单位

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Yokohama City Institute of Health, 1-2-17 Takigashira, Isogo-ku, Yokohama-shi, Kanagawa 235-0012, Japan;

    Chiba City Institute of Health and Environment, 1-3-9 Saiwai-cho, Mihama-ku, Chiba-shi, Chiba 261-0001, Japan;

    Sapporo City Institute of Public Health, 9-1 Kikusui, Shiroishi-ku, Sapporo-shi, Hokkaido 003-8505, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

    Chiba University Graduate School of Engineering, 1-33 Yayoicho, Inage-ku, Chiba-shi, Chiba 263-8522, Japan;

    Department of Environmental Health, National Institute of Public Health, 2-3-6 Minami, Wako-shi, Saitama 351-0197, Japan;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Indoor air quality; Nationwide survey; Diffusive sampler; Ozone;

    机译:室内空气质量全国范围内的调查;扩散取样器;臭氧;

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