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首页> 外文期刊>Environmental Science & Technology >Porous Eleocharis@MnPE Layered Hybrid for Synergistic Adsorption and Catalytic Biodegradation of Toxic Azo Dyes from Industrial Wastewater
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Porous Eleocharis@MnPE Layered Hybrid for Synergistic Adsorption and Catalytic Biodegradation of Toxic Azo Dyes from Industrial Wastewater

机译:多孔Eleocharis @ MnPE层状杂种用于工业废水中有毒偶氮染料的协同吸附和催化生物降解

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摘要

The effective treatment of industrial wastewater to protect freshwater reserves for the survival of life is a primary focus of current research. Herein, a multicomponent Eleocharis-manganese peroxidase enzyme (Eleocharis@MnPE) layered hybrid with high surface area (1200 m(2)/m(3)), with a strong synergistic adsorption and catalytic biodegradation (SACB), has been developed through a facile method. A combination of outer porous (Eleocharis) and inner catalytically active (MnPE) components of the hybrid resulted in highly efficient SACB system, evidenced by high removal rate of 15 kg m(-3) day(-1) (100%) and complete degradation of toxic Orange II (OR) azo dye into nontoxic products (gases and weak acids). The Eleocharis@MnPE layered hybrid efficiently degraded both OR in synthetic wastewater and also other azo dyes (red, pink, and yellow dyes) present in three different textile industrial effluents. For the industrial effluents, these were evidenced by the color disappearance and reduction in biological oxygen demand (BOD), chemical oxygen demand (COD), and total organic carbon (TOC) of up to 97%, 92%, and 76%, respectively. Furthermore, reduced toxicity of treated wastewater was confirmed by decreased cell toxicity to 0.1%-1% and increased cell viability to 90%. We believe that designing a hybrid system with strong ability of SACB could be highly effective for industrial-scale treatment of wastewater.
机译:有效处理工业废水以保护淡水储备以维持生命是当前研究的主要重点。在这里,已经开发了具有高表面积(1200 m(2)/ m(3)),具有强大的协同吸附和催化生物降解作用(SACB)的多组分Eleocharis-锰过氧化物酶(Eleocharis @ MnPE)层状杂种。简便的方法。杂种的外部多孔(Eleocharis)和内部催化活性(MnPE)组分的组合产生了高效的SACB系统,其高去除率达到15 kg m(-3)day(-1)(100%)且完全将有毒的Orange II(OR)偶氮染料降解为无毒产品(气体和弱酸)。 Eleocharis @ MnPE层状杂种可以有效降解合成废水中的OR,还可以降解三种纺织工业废水中存在的其他偶氮染料(红色,粉红色和黄色染料)。对于工业废水,颜色消失和生物需氧量(BOD),化学需氧量(COD)和总有机碳(TOC)减少分别高达97%,92%和76%证明了这一点。 。此外,通过将细胞毒性降低至0.1%-1%和将细胞活力提高至90%,可以确认处理后废水的毒性降低。我们认为,设计具有强大SACB能力的混合系统可能对工业规模的废水处理非常有效。

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  • 来源
    《Environmental Science & Technology》 |2019年第4期|2161-2170|共10页
  • 作者单位

    Univ Agr Faisalabad, Dept Struct & Environm Engn, Faisalabad 38040, Punjab, Pakistan|Peking Univ, Dept Environm Engn, Key Lab Water & Sediment Sci, Minist Educ, Beijing 100871, Peoples R China;

    Univ Agr Faisalabad, Dept Chem, Faisalabad 38040, Punjab, Pakistan;

    Univ Agr Faisalabad, Dept Struct & Environm Engn, Faisalabad 38040, Punjab, Pakistan;

    Univ Agr Faisalabad, Dept Chem, Faisalabad 38040, Punjab, Pakistan;

    South Univ Sci & Technol, Dept Phys, Shenzhen 518055, Peoples R China;

    Natl Ctr Nanosci & Technol, CAS Ctr Excellence Nanosci, CAS Key Lab Standardizat & Measurement Nanotechno, CAS Key Lab Biol Effects Nanomat & Nanosafety, Beijing 100190, Peoples R China;

    Univ Elect Sci & Technol, Sch Mat & Energy, Natl Engn Res Ctr Elect Radiat Control Mat, Ctr Appl Chem, Chengdu 611731, Sichuan, Peoples R China;

    UNSW, Sch Chem Engn, Kensington, NSW 2052, Australia;

    RMIT Univ, Sch Engn, 124 La Trobe St, Melbourne, Vic 3001, Australia;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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