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首页> 外文期刊>Environmental Science & Technology >Atmospheric Occurrence of Legacy Pesticides, Current Use Pesticides, and Flame Retardants in and around Protected Areas in Costa Rica and Uganda
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Atmospheric Occurrence of Legacy Pesticides, Current Use Pesticides, and Flame Retardants in and around Protected Areas in Costa Rica and Uganda

机译:哥斯达黎加和乌干达保护区及其周围地区遗留的传统农药,目前使用的农药和阻燃剂的大气发生

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摘要

Protected areas have developed alongside intensive changes in land use and human settlements in the neighboring landscape. Here, we investigated the occurrence of 21 organochlorine pesticides (OCPs), 14 current use pesticides (CUPs), 47 halogenated flame retardants (HFRs), and 19 organophosphate esters (OPEs) in air around Las Cruces (LC) and La Selva (LS) Biological Stations, Costa Rica, and Kibale National Park (KNP), Uganda using passive air samplers (PAS) with polyurethane foam (PUF) discs (PAS-PUF). Significantly higher concentrations of CUPs were observed around LS, while LC had a higher concentration of OCPs. Land use analysis indicated that LS had a higher fraction of agriculture than LC (33% vs 14%), suggesting the higher CUPs concentration at LS was related to pesticide intensive crops, while higher OCPs concentration at LC may be attributed to the area's long agricultural history characterized by small-scale subsistence farming or long-range transport. In Uganda, CUPs and OCPs were generally lower than in Costa Rica, but high concentrations of HFRs were observed inside KNP, possibly due to human activity at research camps near the protected forest. This is the first study that documented the occurrence of anthropogenic chemicals in the air at protected areas with tropical forests.
机译:保护区的发展与周边景观中土地利用和人类住区的剧烈变化并存。在这里,我们调查了Las Cruces(LC)和La Selva(LS)周围空气中21种有机氯农药(OCP),14种当前使用的农药(CUPs),47种卤化阻燃剂(HFRs)和19种有机磷酸酯(OPEs)的发生情况)哥斯达黎加和乌干达的基巴莱国家公园(KNP)的生物站使用带有聚氨酯泡沫(PUF)盘(PAS-PUF)的被动空气采样器(PAS)。在LS周围观察到明显更高的CUP浓度,而LC则具有更高的OCP浓度。土地利用分析表明,LS的农业比例高于LC(33%比14%),这表明LS的CUP浓度较高与农药密集型作物有关,而LC的OCPs浓度较高可能是由于该地区农业长以小规模自给农业或远距离运输为特征的历史。在乌干达,CUP和OCP普遍低于哥斯达黎加,但在KNP内部观察到高浓度的HFR,这可能是由于保护林附近研究营地的人类活动所致。这是第一项研究记录了热带森林保护区空气中人为化学物质的发生。

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  • 来源
    《Environmental Science & Technology》 |2019年第11期|6171-6181|共11页
  • 作者单位

    Indiana Univ, Sch Publ & Environm Affairs, Bloomington, IN 47405 USA;

    Indiana Univ, Dept Anthropol, Bloomington, IN 47405 USA;

    Indiana Univ, Sch Publ & Environm Affairs, Bloomington, IN 47405 USA;

    Indiana Univ, Dept Anthropol, Bloomington, IN 47405 USA;

    Org Trop Studies, Las Cruces Biol Field Stn, San Vito, Costa Rica;

    MUBFS, Kibale Natl Pk, Ft Porta, Uganda;

    Indiana Univ, Dept Anthropol, Bloomington, IN 47405 USA;

    Indiana Univ, Sch Publ & Environm Affairs, Bloomington, IN 47405 USA;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
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