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首页> 外文期刊>Environmental Science & Technology >Mixing State and Fractal Dimension of Soot Particles at a Remote Site in the Southeastern Tibetan Plateau
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Mixing State and Fractal Dimension of Soot Particles at a Remote Site in the Southeastern Tibetan Plateau

机译:藏藏高原遥控场地烟灰颗粒的混合状态和分形维数

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摘要

The mixing state and fractal dimension (D-f) of soot particles are two major factors affecting their absorption capacity and their climate effects. Here we investigated these factors of soot particles found in a typical valley of the southeastern Tibetan Plateau where wood burning in local villages was one major source of soot particles. Our motivation revealed D-f and the aging property of soot particles in remote air and discussed their regional climatic implications. We found that 64% of total analyzed particles by number were soot-bearing particles and most of them aged with sulfate or organic coating. The D-f sequence is bare-like soot (1.75 +/- 0.08) partly coated soot (1.82 +/- 0.05) embedded soot (1.88 +/- 0.05). The aging process enlarged the overall size of the soot-bearing particles and increased the compactness of soot. Soot aging critically depended on high relative humidity (RH) during nighttime. Besides emission sources and coating processes, the coating aerosol phase under different RHs is another important factor affecting the soot D-f.
机译:烟灰颗粒的混合状态和分形维数(D-F)是影响其吸收能力及其气候效应的两个主要因素。在这里,我们调查了在藏藏高原典型谷中发现的烟灰颗粒的这些因素,其中在当地村庄的木材燃烧是烟灰粒子的一个主要来源。我们的动机揭示了遥远空气中烟灰粒子的D-F和探讨了其区域气候影响。我们发现,通过数量的64%的分析颗粒是含有烟灰的颗粒,其中大部分用硫酸盐或有机涂层变老。 D-F序列是裸露的烟灰(1.75 +/- 0.08)<部分涂层烟灰(1.82 +/- 0.05)<嵌入式烟灰(1.88 +/- 0.05)。老化过程扩大了煤壳颗粒的总体尺寸并增加了烟灰的紧凑性。烟灰老化在夜间期间依赖于高相对湿度(RH)。除了发射源和涂布过程之外,不同RH下的涂层气溶胶相是影响烟灰D-F的另一个重要因素。

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  • 来源
    《Environmental Science & Technology》 |2019年第14期|8227-8234|共8页
  • 作者单位

    Zhejiang Univ Sch Earth Sci Dept Atmospher Sci Hangzhou 310027 Zhejiang Peoples R China;

    Chinese Acad Sci Northwest Inst Ecoenvironm & Resources State Key Lab Cryospher Sci Lanzhou 730000 Gansu Peoples R China;

    Zhejiang Univ Sch Earth Sci Dept Atmospher Sci Hangzhou 310027 Zhejiang Peoples R China;

    Chinese Acad Sci Northwest Inst Ecoenvironm & Resources State Key Lab Cryospher Sci Lanzhou 730000 Gansu Peoples R China;

    Zhejiang Univ Sch Earth Sci Dept Atmospher Sci Hangzhou 310027 Zhejiang Peoples R China;

    Zhejiang Univ Sch Earth Sci Dept Atmospher Sci Hangzhou 310027 Zhejiang Peoples R China;

    Zhejiang Univ Sch Earth Sci Dept Atmospher Sci Hangzhou 310027 Zhejiang Peoples R China;

    Chinese Acad Sci Northwest Inst Ecoenvironm & Resources State Key Lab Cryospher Sci Lanzhou 730000 Gansu Peoples R China|CAS Ctr Excellence Tibetan Plateau Earth Sci Beijing 100101 Peoples R China;

    Zhejiang Univ Sch Earth Sci Dept Atmospher Sci Hangzhou 310027 Zhejiang Peoples R China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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  • 正文语种 eng
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