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首页> 外文期刊>Environmental Science & Technology >Anthropogenic Osmium in Macroalgae from Tokyo Bay Reveals Widespread Contamination from Municipal Solid Waste
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Anthropogenic Osmium in Macroalgae from Tokyo Bay Reveals Widespread Contamination from Municipal Solid Waste

机译:来自东京湾大理石藻类的人为锇揭示了城市固体废物的广泛污染

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摘要

Human activity is influencing the global osmium cycle, driving the Os isotopic composition (~(187)Os/~(188)Os) of the hydrosphere and associated sedimentary material to lower values. Here, we present the Re and Os abundance and isotope systematics of macroalgae, a proxy for seawater, from Tokyo Bay to elucidate the potential sources of anthropogenic Os to the Pacific Ocean. Macroalgae from the Uraga Channel, which connects Tokyo Bay to the Pacific Ocean, record relatively low Os abundances (~10.1 pg/ g) and an ~(187)Os/~(188)Os of ~0.9, indicative of surface ocean seawater. Contrastingly, macroalgae within the bay closest to central Tokyo record the highest Os abundances (~22.8 pg/g) and lowest ~(187)Os/~(188)Os values (~0.47), suggesting contamination from human activity. To determine the source of anthropogenic Os, we have developed the first Os emission inventory, based on the East Asian Air Pollutant Emission Grid database (EAGrid2010). The close relationship (R~2 = 0.67 and p-value = <0.05) between Os inventories and macroalgal data suggests that municipal solid waste incinerators (MSWIs) are the dominant source of Os to Tokyo Bay. Projections for Japan estimate that 26_(18)~(38) ng Os/m~2/yr is released from MSWI smokestacks, leading to a concentration in precipitation of 26_(18)~(38) fg/g, identifying MSWIs as a major contributor of anthropogenic Os to the hydrological cycle.
机译:人类活动正在影响全局锇循环,驱动卫生间同位素组合物(〜(187)OS /〜(188)OS)的水层和相关沉积物以降低值。在这里,我们介绍了大型宏观的Re和Os丰度和同位素系统,来自东京海湾的海水代理,阐明了太平洋的人为OS的潜在来源。来自Uraga频道的巨大峡谷,将东京湾连接到太平洋,纪录相对低的OS丰度(〜10.1 pg / g)和〜(187)OS /〜(188)OS〜0.9,表示表面海洋海水。比较的是,海湾内的宏观格盖最接近东京中央丰富(〜22.8 pg / g)和最低〜(187)OS /〜(188)OS值(〜0.47),暗示人类活动污染。为了确定人为OS的来源,我们已经开发了基于东亚空气污染物发射网格数据库(EAGRID2010)的第一个OS排放清单。 OS清单与宏观数据之间的密切关系(R〜2 = 0.67和p值= <0.05)表明市政固体废物焚烧炉(MSWIS)是东京湾的主导源。日本的预测估计26_(18)〜(38)NG OS / M〜2 / YR从MSWI烟囊中释放,导致沉淀的浓度为26_(18)〜(38)FG / g,识别Mswis作为一个人为OS对水文循环的主要贡献者。

著录项

  • 来源
    《Environmental Science & Technology》 |2020年第15期|9356-9365|共10页
  • 作者单位

    Department of Earth Sciences Durham University Durham DH1 3LE U.K. Atmosphere and Ocean Research Institute The University of Tokyo Chiba 263-0022 Japan;

    Department of Earth Sciences Durham University Durham DH1 3LE U.K. State Key Laboratory of Geological Processes and Mineral Resources School of Earth Resources China University of Geosciences Wuhan 430074 Hubei China;

    Submarine Resources Research Center JAMSTEC Yokosuka 237-0061 Japan;

    Global Modelling and Assimilation Office NASA Goddard Space Flight Center Greenbelt 20771 Maryland United States Goddard Earth Sciences Technology and Research Universities Space Research Association Columbia 21046-2132 Maryland United States;

    Atmosphere and Ocean Research Institute The University of Tokyo Chiba 263-0022 Japan;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
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