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Release of Plastics to Australian Land from Biosolids End-Use

机译:从Biosolids最终用途释放塑料到澳大利亚土地

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摘要

Plastics are contaminants of emerging concern that can enter the environment from multiple sources, including via land application of treated sewage sludge (biosolids). Biosolids samples collected from 82 wastewater treatment plants (WWTPs) across Australia and covering 34% of the population during census week in 2016 were quantitatively analyzed to estimate the release of seven common plastics. Quantitative analysis was performed by pressurized liquid extraction followed by double-shot microfurnace pyrolysis coupled to gas chromatography mass spectrometry. Ninety nine percent of the samples contained plastics (Σ_6plastics) at concentrations of between 0.4 and 23.5 mg/g dry weight (median; 10.4 mg/g dry weight), while polycarbonate was not detected in any sample. Per-capita mass loads of plastics (Σ_6plastics) released were between 8 and 877 g/person/year across all investigated WWTPs. Polyethylene was the predominant plastic detected, contributing to 69% of Σ_6plastics. Based on the concentrations measured, it was projected that around 4700 metric tons (Mt) of plastics are released into the Australian environment through biosolids end-use each year, equating to approximately 200 g/person/ year, which represents 0.13% of total plastics use in Australia. Of this, 3700 Mt of plastics are released to agricultural lands and 140 Mt to landscape topsoil. Our results provide a first quantitative per-capita mass loads and emission estimate of plastic types through biosolids end-use.
机译:塑料是新兴担心的污染物,可以从多种来源进入环境,包括经过处理过的污水污泥(Biosolids)的土地应用。在澳大利亚的82个废水处理厂(WWTPS)中收集的Biosolids样品,并在2016年人口普查周内占据了34%的人口,以定量分析,以估计七种常见塑料的释放。通过加压液体萃取进行定量分析,然后进行双滴微覆盖热解,偶联至气相色谱质谱法。在0.4和23.5mg / g干重(中位数; 10.4mg / g干重)的浓度下含有百分之九十九十个样品含有塑料(σα6plastics),而在任何样品中未检测到聚碳酸酯。释放的塑料(σ_6plastics)的人均大众荷载量在所有调查的WWTPS中释放的8至877克/年介于877克/年之间。聚乙烯是检测到的主要塑料,有助于69%的σ_6plastics。基于测量的浓度,预计将通过每年的生物溶解于每年使用的生物溶解率约为4700公吨(MT),等于约200克/人/年,占总塑料的0.13%在澳大利亚使用。其中,3700吨塑料被释放到农业土地和140公吨景观表土。我们的结果通过生物溶解的最终用途提供了第一种定量的人均大规模载荷和塑料类型的排放估计。

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  • 来源
    《Environmental Science & Technology》 |2020年第23期|15132-15141|共10页
  • 作者单位

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia College of Life and Environmental Sciences University of Exeter Exeter EX4 4QD U.K.;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia College of Life and Environmental Sciences University of Exeter Exeter EX4 4QD U.K.;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

    Queensland Alliance for Environmental Health Sciences (QAEHS) The University of Queensland Woolloongabba Queensland 4102 Australia;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
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