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首页> 外文期刊>Environmental Science & Technology >Spatial and Seasonal Distributions of Current Use Pesticides (CUPs) in the Atmospheric Particulate Phase in the Great Lakes Region
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Spatial and Seasonal Distributions of Current Use Pesticides (CUPs) in the Atmospheric Particulate Phase in the Great Lakes Region

机译：大湖区大气颗粒相中当前使用农药的空间和季节分布

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摘要

The authors analyzed spatial and seasonal variations of current use pesticides (CUPs) levels in the atmospheric particulate phase in the Great Lakes basin. Twenty-four hour air samples were collected at six sites (two urban, two rural, and two remote) in 2015. The concentrations of 15 CUPs, including nine pyrethroid insecticides, four herbicides, one organophosphate insecticide, and one fungicide, were measured. The total CUPs concentrations were higher at the urban sites (0.38–1760 pg/m~(3)) than at the rural and remote sites (0.07–530 pg/m~(3)). The most abundant CUPs were pyrethroid insecticides at the urban sites. The levels of the other CUPs did not vary much among the six sites, except at the most remote site at Eagle Harbor, where the levels were significantly lower. Chlorothalonil was the most frequently detected CUP, which was detected in more than 76% of the samples. The atmospheric concentrations of total pyrethroid insecticides and total herbicides were correlated with local human population and developed land use. Significantly higher concentrations of most CUPs were observed in the warmer months than in the colder months at all sites. In addition to agricultural applications, which occur during the warmer months, the CUPs atmospheric concentrations may also be influenced by nonagricultural activities and the urban development.
机译：作者分析了大湖流域大气颗粒相中当前使用农药（CUPs）水平的时空变化。 2015年，在六个地点（两个城市，两个农村和两个偏远地区）收集了24小时的空气样本。测量了15个CUP的浓度，其中包括9种拟除虫菊酯类杀虫剂，4种除草剂，一种有机磷杀虫剂和一种杀真菌剂。城市地区的CUPs总浓度（0.38-1760 pg / m〜（3））高于农村和偏远地区的0.07-530 pg / m〜（3）。在城市地区，最丰富的银联农药是拟除虫菊酯类杀虫剂。在六个站点中，其他CUP的级别变化不大，除了鹰港最偏远的站点外，其级别明显较低。氯噻酮是最常检测到的CUP，在超过76％的样品中被检测到。拟除虫菊酯类杀虫剂和除草剂总量的大气浓度与当地人口和发达的土地利用相关。在所有地点，在较温暖的月份观察到的大多数CUP的浓度明显高于较寒冷的月份。除了在较温暖的月份发生的农业应用外，银联的大气浓度还可能受到非农业活动和城市发展的影响。

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  • 来源
    《Environmental Science & Technology》 |2018年第11期|6177-6186|共10页
  • 作者

    Shaorui Wang; Amina Salamova; Ronald A. Hites; Marta Venier;

  • 作者单位

    School of Public and Environmental Affairs, Indiana University, Bloomington, Indiana 47405, United States;

    School of Public and Environmental Affairs, Indiana University, Bloomington, Indiana 47405, United States;

    School of Public and Environmental Affairs, Indiana University, Bloomington, Indiana 47405, United States;

    School of Public and Environmental Affairs, Indiana University, Bloomington, Indiana 47405, United States;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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  • 正文语种 eng
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