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首页> 外文期刊>Environmental Science & Technology >Geographical Differences in Dietary Exposure to Perfluoroalkyl Acids between Manufacturing and Application Regions in China
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Geographical Differences in Dietary Exposure to Perfluoroalkyl Acids between Manufacturing and Application Regions in China

机译：中国生产和应用地区之间全氟烷基酸饮食暴露的地理差异

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摘要

Emissions of perfluoroalkyl acids (PFAAs) have increased in China over the past decade, but human exposure pathways are poorly understood. Here we analyzed 15 PFAAs in commonly consumed food items and calculated body weight normalized dietary intake rates (estimated dietary intake, EDIs) in an area with ongoing PFAA production (Hubei province; n = 121) and an urbanized coastal area (Zhejiang province； n = 106). Geographical differences in concentrations were primarily observed for perfluorooctanesulfonic acid (PFOS) and perfluorohexanesnlfonic acid (PFHxS) in animal food items and short-chain PFAAs in vegetable food items. The average EDI of ΣPFAAs for adults in Hubei (998 ng kg~(-1) day~(-1) was more than 2 orders of magnitude higher than that in Zhejiang (9.03 ng kg~(-1) day~(-1). In Hubei province, the average EDI of PFOS for adults (87 ng kg~(-1) day~(-1)) was dose to or exceeded advisory guidelines used in other countries indicating health risks for the population from long-term exposure. Yet, PFOS could only account for about 10% of the EDI of ΣPFAAs in the Hubei province, which was dominated by short-chain PFAAs through consumption of vegetables. The large contribution of short-chain PFAAs to the total EDIs in manufacturing areas emphasize the need for improved exposure and hazard assessment tools of these substances.
机译：在过去的十年中，中国的全氟烷基酸（PFAA）排放量有所增加，但是人们对人体的暴露途径知之甚少。在这里，我们分析了PFAA持续生产地区（湖北省； n = 121）和城市化沿海地区（浙江省； n）的15种常见食用食品中的PFAA，并计算了体重标准化饮食摄入率（估计饮食摄入量，EDI）。 = 106）。主要观察到动物食品中全氟辛烷磺酸（PFOS）和全氟己烷磺酸（PFHxS）以及蔬菜食品中短链PFAAs浓度的地理差异。湖北（998 ng kg〜（-1）天〜（-1）成年人的ΣPFAA的平均EDI比浙江的9.03 ng kg〜（-1）天〜（-1）高2个数量级以上。 ）。在湖北省，成年人的全氟辛烷磺酸平均EDI（87 ng kg〜（-1）天〜（-1））达到或超过了其他国家/地区使用的咨询准则，表明长期人口对健康的危害然而，全氟辛烷磺酸仅占湖北省ΣPFAA的EDI的10％左右，而短链PFAA则通过食用蔬菜而占主导地位，而短链PFAA对制造业地区EDI总量的贡献很大。强调需要改进这些物质的暴露和危害评估工具。

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  • 来源
    《Environmental Science & Technology》 |2017年第10期|5747-5755|共9页
  • 作者

    Haiyan Zhang; Robin Vestergren; Thanh Wang; Junchao Yu; Guibin Jiang; Dorte Herzke;

  • 作者单位

    College of Environment, Zhejiang University of Technology, Hangzhou 310032, China,State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China;

    Norwegian Institute for Air Research (NILU), FRAM - High North Research Centre on Climate and the Environment, Tromsø, Norway,ACES - Department of Environmental Science and Analytical Chemistry, Stockholm University, Stockholm, Sweden;

    MTM Research Centre, School of Science and Technology, Örebro University, Örebro, Sweden;

    ,Norwegian Institute for Air Research (NILU), FRAM - High North Research Centre on Climate and the Environment, Tromsø, Norway;

    State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China;

    State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China;

    Norwegian Institute for Air Research (NILU), FRAM - High North Research Centre on Climate and the Environment, Tromsø, Norway;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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