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Aircraft-Based Estimate of Total Methane Emissions from the Barnett Shale Region

机译:基于飞机的巴尼特页岩地区甲烷排放总量估算

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摘要

We present estimates of regional methane (CH_4) emissions from oil and natural gas operations in the Barnett Shale, Texas, using airborne atmospheric measurements. Using a mass balance approach on eight different flight days in March and October 2013, the total CH_4 emissions for the region are estimated to be 76 ± 13 × 10~3 kg hr~(-1) (equivalent to 0.66 ± 0.11 Tg CH_4 yr~(-1); 95% confidence interval (CI)). We estimate that 60 ± 11 × 10~3 kg CH_4 hr~(-1) (95% CI) are emitted by natural gas and oil operations, including production, processing, and distribution in the urban areas of Dallas and Fort Worth. This estimate agrees with the U.S. Environmental Protection Agency (EPA) estimate for nationwide CH_4 emissions from the natural gas sector when scaled by natural gas production, but it is higher than emissions reported by the EDGAR inventory or by industry to EPA's Greenhouse Gas Reporting Program. This study is the first to show consistency between mass balance results on so many different days and in two different seasons, enabling better quantification of the related uncertainty. The Bamett is one of the largest production basins in the United States, with 8% of total U.S. natural gas production, and thus, our results represent a crucial step toward determining the greenhouse gas footprint of U.S. onshore natural gas production.
机译:我们使用大气中的大气测量值,估算了得克萨斯州Barnett页岩中石油和天然气运营产生的区域甲烷(CH_4)排放量。使用质量平衡方法,在2013年3月和10月的8个不同的飞行日,该地区的CH_4排放总量估计为76±13×10〜3 kg hr〜(-1)(相当于0.66±0.11 Tg CH_4 yr) 〜(-1); 95%置信区间(CI))。我们估计,天然气和石油运营,包括达拉斯和沃思堡市区的生产,加工和分销,排放的甲烷为60±11×10〜3 kg CH_4 hr〜(-1)(95%CI)。此估算值与美国环境保护署(EPA)估算的天然气产量在全国范围内的CH_4排放量相符,但高于EDGAR清单或行业向EPA温室气体报告计划报告的排放量。这项研究是第一个显示这么多不同的天数和两个不同的季节中质量平衡结果之间一致性的方法,从而可以更好地量化相关不确定性。 Bamett是美国最大的生产盆地之一,占美国天然气总产量的8%,因此,我们的结果代表了确定美国陆上天然气生产的温室气体足迹的关键一步。

著录项

  • 来源
    《Environmental Science & Technology》 |2015年第13期|8124-8131|共8页
  • 作者单位

    University of Colorado, CIRES, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    University of Colorado, CIRES, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    University of Michigan, Ann Arbor, Michigan 48109, United States;

    Purdue University, West Lafayette, Indiana 47907, United States;

    NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    Purdue University, West Lafayette, Indiana 47907, United States,Ateneo de Manila University, Quezon City, Philippines;

    University of California, Davis, Davis, California 95616, United States;

    Carbon Now Cast, LLC, State College, Pennsylvania 16803, United States;

    Carbon Now Cast, LLC, State College, Pennsylvania 16803, United States;

    University of Colorado, CIRES, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    Aerodyne Research, Inc., Billerica, Massachusetts 01821, United States;

    Carbon Now Cast, LLC, State College, Pennsylvania 16803, United States;

    Purdue University, West Lafayette, Indiana 47907, United States;

    Environmental Defense Fund, Austin, Texas 78701, United States;

    University of Colorado, CIRES, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    University of Colorado, CIRES, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    Picarro, Inc., Santa Clara, California 95054, United States;

    University of Michigan, Ann Arbor, Michigan 48109, United States;

    University of Colorado, CIRES, Boulder, Colorado 80309, United States,NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

    Aerodyne Research, Inc., Billerica, Massachusetts 01821, United States;

    NOAA Earth System Research Laboratory, Boulder 80305, Colorado, United States;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
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