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Occurrence and Distribution of Disinfection Byproducts in Domestic Wastewater Effluent, Tap Water, and Surface Water during the SARS-CoV-2 Pandemic in China

机译:中国苏格兰州SARS-COV-2大流行病中,在国内废水污水,自来水和地表水中消毒副产品的发生和分布

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摘要

Intensified efforts to curb transmission of the Severe Acute Respiratory Syndrome Coronavirus-2 might lead to an elevated concentration of disinfectants in domestic wastewater and drinking water in China, possibly resulting in the generation of numerous toxic disinfection byproducts (DBPs). In this study, the occurrence and distribution of five categories of DBPs, including six trihalomethanes (THMs), nine haloacetic acids (HAAs), two haloketones, nine nitrosamines, and nine aromatic halogenated DBPs, in domestic wastewater effluent, tap water, and surface water were investigated. The results showed that the total concentration level of measured DBPs in wastewater effluents (78.3 μg/L) was higher than that in tap water (56.0 μg/L, p = 0.05), followed by surface water (8.0 μg/L, p < 0.01). Moreover, HAAs and THMs were the two most dominant categories of DBPs in wastewater effluents, tap water, and surface water, accounting for >90%, respectively. Out of the regulated DBPs, none of the wastewater effluents and tap water samples exceeded the corresponding maximum guideline values of chloroform (300 μg/L), THM4 (80 μg/L), NDMA (100 ng/L), and only 2 of 35 tap water samples (67.6 and 63.3 μg/L) exceeded the HAA5 (60 μg/L) safe limit. HAAs in wastewater effluents showed higher values of risk quotient for green algae. This study illustrates that the elevated use of disinfectants within the guidance ranges during water disinfection did not result in a significant increase in the concentration of DBPs.
机译:强烈努力抑制严重急性呼吸综合征冠状病毒-2的传播可能导致在中国国内废水和饮用水中升高的消毒剂,可能导致多种毒性消毒副产品(DBPS)。在本研究中,五类DBP的发生和分布,包括六个三卤甲烷(THM),九卤代乙酸(HAAs),两种卤代酮,九个亚硝胺和九个芳香卤化DBPS,在国内废水流出物中,自来水和表面调查了水。结果表明,废水流出物中测量的Dbps的总浓度水平高于自来水(56.0μg/ L,P = 0.05),然后是地表水(8.0μg/ L,P < 0.01)。此外,HAAS和THM是废水污水,自来水和地表水中的两种最主导的DBP类别,分别占> 90%。从受调节的DBPS中,没有废水流出物和自来水样品超过氯仿(300μg/ L),THM4(80μg/ L),NDMA(100ng / L)的最大准则值,只有2个35自来水样品(67.6和63.3μg/ L)超过HAA5(60μg/ L)安全限制。废水污水中的HAAs显示出绿藻的风险商值较高。本研究表明,在水消毒过程中,在引导范围内升高的消毒剂的使用并未导致Dbps浓度的显着增加。

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  • 来源
    《Environmental Science & Technology》 |2021年第7期|4103-4114|共12页
  • 作者单位

    School of Environment Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences Hangzhou 310000 People's Republic of China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 10008S People's Republic of China;

    State Key Laboratory of Freshwater Ecology and Biotechnology Institute of Hydrobiology Chinese Academy of Sciences Wuhan 430072 People's Republic of China;

    State Key Laboratory of Freshwater Ecology and Biotechnology Institute of Hydrobiology Chinese Academy of Sciences Wuhan 430072 People's Republic of China;

    State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 People's Republic of China;

    State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 People's Republic of China;

    State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 People's Republic of China;

    School of Environment Hangzhou Institute for Advanced Study and University of Chinese Academy of Sciences Hangzhou 310000 People's Republic of China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 People's Republic of China;

    State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 People's Republic of China;

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  • 正文语种 eng
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