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首页> 外文期刊>Environmental Science & Technology >Polybrominated Diphenyl Ethers, 2,2',4,4',5,5'-Hexachlorobiphenyl (PCB-153), and p,p'-Dichlorodiphenyldichloroethylene (p,p'-DDE) Concentrations in Sera Collected in 2009 from Texas Children
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Polybrominated Diphenyl Ethers, 2,2',4,4',5,5'-Hexachlorobiphenyl (PCB-153), and p,p'-Dichlorodiphenyldichloroethylene (p,p'-DDE) Concentrations in Sera Collected in 2009 from Texas Children

机译:2009年从得克萨斯州儿童处收集的血清中的多溴联苯醚,2,2',4,4',5,5'-六氯联苯(PCB-153)和p,p'-二氯二苯基二氯乙烯(p,p'-DDE)浓度

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摘要

Polybrominated diphenyl ethers (PBDEs), polychlorinated biphen- yls (PCBs) and p,p'-dichlorodiphenyldichloroethylene (p,p'-DDE) have been measured in surplus serum collected in 2009 from a convenience sample of 300 Texas children (boys and girls) in the birth to 13 years of age range. Serum concentrations of traditional persistent organic pollutants such as 2,2',4,4',5,5'- hexachlorobiphenyl (PCB-153) and p,p'-DDE did not change consistently with age. By contrast, serum concentrations of terra-, penta-, and hexa-BDEs were lowest in the youngest children (birth to two year old) and increased 3.0 to 7.9 times, depending on the analyte, for children in the >4 to 6 years of age group. From the apex concentration to the 10 to 13 years of age group, concentrations decreased significantly except for 2,2',4,4',5,5'-hexabromodiphenyl ether (PBDE- 153), which also had a longer apex concentration of >4 to 8 years of age. This concentration trend for PBDE-153 is most likely due to a longer half-life of PBDE- 153 than of other PBDE congeners. The observed PBDEs concentration patterns by age may be related, at least in part, to ingestion of residential dust containing PBDEs through hand-to-mouth behavior among toddlers, preschoolers, and kindergarteners. Further studies to characterize young children's exposure to PBDEs are warranted and, in particular, to determine the lifestyle factors that may contribute to such exposures.
机译:2009年从300名得克萨斯州儿童(男童和女童)的便利样本中收集了多余血清中的多溴联苯醚(PBDEs),多氯联苯(PCBs)和对苯二酚(p,p'-dichlorodiphenyldichloroethylene(p,p'-DDE))。 )出生至13岁以下。传统的持久性有机污染物如2,2',4,4',5,5'-六氯联苯(PCB-153)和p,p'-DDE的血清浓度不会随年龄而变化。相比之下,年龄最小(出生至两岁)的儿童中血清六溴二苯醚,五溴二苯醚和六溴二苯醚的浓度最低,对于4至6岁的儿童,视分析物而定,增加了3.0至7.9倍年龄组。从顶点浓度到10至13岁年龄段,浓度显着下降,除了2,2',4,4',5,5'-六溴二苯醚(PBDE-153),后者的顶点浓度也更长。 > 4至8岁。 PBDE-153的这种浓度趋势最可能是由于PBDE-153的半衰期比其他PBDE同类物更长。观察到的按年龄划分的多溴二苯醚浓度模式可能至少部分与通过幼儿,学龄前儿童和幼稚园儿童的口口行为摄入含有多溴二苯醚的住宅灰尘有关。有必要进行进一步的研究以表征幼儿对多溴二苯醚的接触,特别是确定可能导致这种接触的生活方式因素。

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  • 来源
    《Environmental Science & Technology》 |2014年第14期|8196-8202|共7页
  • 作者单位

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    School of Public Health, University of Texas Dallas Regional Campus, 6011 Harry Hines Boulevard V8.112, Dallas, Texas 75390, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    School of Public Health, University of Michigan, 1415 Washington Heights, Ann Arbor, Michigan 48109, United States;

    School of Public Health, University of Texas Dallas Regional Campus, 6011 Harry Hines Boulevard V8.112, Dallas, Texas 75390, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

    National Center for Environmental Health, Centers for Disease Control and Prevention, 4770 Buford Highway, Atlanta, Georgia 30341, United States;

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