Transfer of Tritium Released into the Marine Environment by French Nuclear Facilities Bordering the English Channel

Bruno Fievet; Julien Pommier; Claire Voiseux; Pascal Bailly du Bois; Philippe Laguionie; Catherine Cossonnet; Luc Solier

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Transfer of Tritium Released into the Marine Environment by French Nuclear Facilities Bordering the English Channel

机译：由与英吉利海峡接壤的法国核设施向海洋环境释放的of的转移

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Controlled amounts of liquid tritium are discharged as tritiated voter (HTO) by the nuclear industry into the English Channel. Because the isotopic discrimination between 3H and H is small, organically bound tritium (OBT) and HTO should show the same T/H ratio under steady-state conditions. We report data collected from the environment in the English Channel. Tritium concentrations measured in seawater HTO, as well as in biota HTO and OBT, confirm that tritium transfers from HTO to OBT result in conservation of the T/H ratio (ca. 1 × 10~(-16)). The kinetics of the turnover of tritium between seawater HTO, biota HTO, and OBT was investigated. HTO in two algae and a mollusk is shown to exchange rapidly with seawater HTO. However, the overall tritium turnover between HTO and the whole-organism OBT is a slow process with a tritium biological half-life on the order of months. Nonsteady-state conditions exist where there are sharp changes in seawater HTO. As a consequence, for kinetic reasons, the T/H ratio in OBT may deviate transiently from that observed in HTO of samples from the marine ecosystem. Dynamic modeling is thus more realistic for predicting tritium transfers to biota OBT under nonsteady-state conditions.

机译：核工业将受控量的液态industry作为as化投票者（HTO）排放到英吉利海峡。由于3H和H之间的同位素分辨力很小，因此在稳态条件下有机结合的tri（OBT）和HTO应该显示出相同的T / H比。我们在英吉利海峡报告从环境中收集的数据。在海水HTO以及生物区系HTO和OBT中测得的concentrations浓度，证实了from从HTO向OBT的转移导致了T / H比的守恒（约1×10〜（-16））。研究了海水HTO，生物区系HTO和OBT之间of的转化动力学。两种藻类和软体动物中的HTO与海水HTO迅速交换。但是，HTO和整个有机物OBT之间的总tri转化是一个缓慢的过程，a生物半衰期约为数月。海水HTO发生急剧变化时，存在非稳态条件。因此，出于动力学原因，OBT中的T / H比可能会暂时偏离海洋生态系统样品的HTO中观察到的T / H比。因此，动态模型对于预测predict在非稳态条件下向生物群OBT的转移更为现实。

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《Environmental Science & Technology》 |2013年第12期|6696-6703|共8页
作者
Bruno Fievet; Julien Pommier; Claire Voiseux; Pascal Bailly du Bois; Philippe Laguionie; Catherine Cossonnet; Luc Solier;
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作者单位

Institut de Radioprotection et de Surete Nucleaire Laboratoire de Radioecologie de Cherbourg-Octeville, IRSN/PRP-ENV/SERIS, Rue Max Pol Fouchet, BP 10, 50130 Cherbourg Octeville, France;

Institut de Radioprotection et de Surete Nucleaire Laboratoire de Radioecologie de Cherbourg-Octeville, IRSN/PRP-ENV/SERIS, Rue Max Pol Fouchet, BP 10, 50130 Cherbourg Octeville, France;

Institut de Radioprotection et de Surete Nucleaire Laboratoire de Radioecologie de Cherbourg-Octeville, IRSN/PRP-ENV/SERIS, Rue Max Pol Fouchet, BP 10, 50130 Cherbourg Octeville, France;

Institut de Radioprotection et de Surete Nucleaire Laboratoire de Radioecologie de Cherbourg-Octeville, IRSN/PRP-ENV/SERIS, Rue Max Pol Fouchet, BP 10, 50130 Cherbourg Octeville, France;

Institut de Radioprotection et de Surete Nucleaire Laboratoire de Radioecologie de Cherbourg-Octeville, IRSN/PRP-ENV/SERIS, Rue Max Pol Fouchet, BP 10, 50130 Cherbourg Octeville, France;

Laboratoire de Mesure de la Radioactivite dans l'Environnement, IRSN/PRP-ENV/STEME, Bois des Rames - Bat 501, 91400 Orsay, France;

Institut de Radioprotection et de Surete Nucleaire Laboratoire de Radioecologie de Cherbourg-Octeville, IRSN/PRP-ENV/SERIS, Rue Max Pol Fouchet, BP 10, 50130 Cherbourg Octeville, France;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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1. Levels of tritium in soils and vegetation near Canadian nuclear facilities releasing tritium to the atmosphere: implications for environmental models [J] . P.A. Thompson, N.-O.A. Kwamena, M. Ilin, Journal of Environmental Radioactivity . 2015,第feba期

机译：加拿大核设施附近土壤和植被中的releasing水平向大气释放tri：对环境模型的影响
2. The TOCATTA-χ model for assessing ~(14)C transfers to grass: an evaluation for atmospheric operational releases from nuclear facilities [J] . Celine Aulagnier, Severine Le Dizes, Denis Maro, Journal of Environmental Radioactivity . 2013,第juna期

机译：评估〜（14）C向草的转移的TOCATTA-χ模型：对核设施大气运行释放的评估
3. Concentration factors and biological half-lives for the dynamic modelling of radionuclide transfers to marine biota in the English Channel [J] . Bruno Fievet, Pascal Bailly du Bois, Claire Voiseux Science of the total environment . 2021,第Octa15期

机译：浓缩因子和生物半衰期，用于辐射核素转移到英语频道海洋生物群的动态建模
4. Model used for assessing the environmental transfer of radionuclides from routine releases of IFIN-HH nuclear facilities [C] . D. Ene Protection of the Environment from the Effects of Ionizing Radiation . 2005

机译：用于评估IFIN-HH核设施常规释放中放射性核素的环境转移的模型
5. Subsecond kinetics of synaptosomal tritium-gamma-aminobutyric acid release, and the relationship to presynaptic calcium(II) channels. [D] . Turner, Timothy John. 1989

机译：突触体tri-γ-氨基丁酸释放的亚秒动力学，以及与突触前钙离子通道的关系。
6. Tritium in the environment from nuclear powerplants. [O] . C. L. Weaver, E. D. Harward, H. T. Peterson Jr 1969

机译：nuclear在环境中来自核电厂。
7. Levels of tritium in soils and vegetation near Canadian nuclear facilities releasing tritium to the atmosphere: implications for environmental models [O] . Thompson P.A., Kwamena N.-O.A., Ilin M., 2015

机译：加拿大核设施附近土壤和植被中的水平向大气释放tri：对环境模型的影响
8. Description of NORMTRI: a computer program for assessing the off-site consequences from air-borne releases of tritium during normal operation of nuclear facilities [R] . Raskob, W. 1994

机译：NORmTRI的描述：一种计算机程序，用于评估核设施正常运行期间空气中氚释放造成的非现场后果

Transfer of Tritium Released into the Marine Environment by French Nuclear Facilities Bordering the English Channel

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