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首页> 外文期刊>Environmental Science & Technology >Indoor Air Is a Significant Source of Tri-decabrominated Diphenyl Ethers to Outdoor Air via Ventilation Systems
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Indoor Air Is a Significant Source of Tri-decabrominated Diphenyl Ethers to Outdoor Air via Ventilation Systems

机译:通过通风系统,室内空气是三十溴化二苯醚向室外空气的重要来源

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摘要

Ventilation of indoor air has been hypothesized to be a source of PBOEs to outdoors. To study this, tri-decabrominated diphenyl ethers were analyzed in outgoing air samples collected inside ventilation systems just before exiting 33 buildings and compared to indoor air samples from microenvironments in each building collected simultaneously. Median Σ_(10)PBDE (BDE- 28, -47, -99, -153, -183, -197, -206, -207, -208, -209) concentrations in air from apartment, office and day care center buildings were 93, 3700, and 660 pg/m~3 for outgoing air, and 92, 4700, and 1200 pg/m~3 for indoor air, respectively. BDE-209 was the major congener found. No statistically significant differences were seen for individual PBDE concentrations in matched indoor and outgoing air samples, indicating that outgoing air PBDE concentrations are equivalent to indoor air concentrations. PBDE concentrations in indoor and outgoing air were higher than published outdoor air values suggesting ventilation as a conduit of PBDEs, including BDE-209, from indoors to outdoors. BDE-209 and sum of BDE-28, -47, -99, and -153 emissions from indoor air to outdoors were roughly estimated to represent close to 90% of total emissions to outdoor air for Sweden, indicating that contaminated indoor air is an important source of PBDE contamination to outdoor air.
机译:假设室内空气的通风是室外PBOE的来源。为了研究这一点,在离开33座建筑物之前,对通风系统内部收集的出风样品中的三十溴化二苯醚进行了分析,并将其与同时从每座建筑物的微环境中收集的室内空气样品进行了比较。公寓,办公室和日托中心大楼空气中的Σ_(10)PBDE(BDE- 28,-47,-99,-153,-183,-197,-206,-207,-208,-209)的中位数浓度出风量分别为93、3700和660 pg / m〜3,室内空气分别为92、4700和1200 pg / m〜3。 BDE-209是发现的主要同类物。在匹配的室内和外出空气样本中,各个PBDE的浓度均未见统计学上的显着差异,这表明外出的PBDE浓度与室内空气浓度相当。室内和流出空气中的PBDE浓度高于公布的室外空气值,表明通风是从室内到室外的多溴二苯醚(包括BDE-209)的管道。 BDE-209以及从室内空气到室外的BDE-28,-47,-99和-153排放物的总和被粗略估计约占瑞典室外空气总排放量的90%,这表明受污染的室内空气是一种PBDE污染室外空气的重要来源。

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  • 来源
    《Environmental Science & Technology》 |2012年第11期|p.5876-5884|共9页
  • 作者单位

    Department of Applied Environmental Science (ITM), Stockholm University, SE-106 91 Stockholm, Sweden;

    Swedish National Heritage Board, Box 1114, 621 22 Visby, Sweden;

    IVL Swedish Environmental Research Institute, Box 21060, SE-10031 Stockholm, Sweden;

    Department of Applied Environmental Science (ITM), Stockholm University, SE-106 91 Stockholm, Sweden;

    Public Health Sciences, Occupational and Environmental Medicine, Karolinska Institutet, Norrbacka, fourth level, SE-17176 Stockholm, Sweden;

    Department of Applied Environmental Science (ITM), Stockholm University, SE-106 91 Stockholm, Sweden;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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  • 正文语种 eng
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