Comment on 'Direct Observation of Tetrahedrally Coordinated Fe(Ⅲ) in Ferrihydrite'

Rosalie K. Hocking; Will P. Gates; John D. Cashion

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Comment on 'Direct Observation of Tetrahedrally Coordinated Fe(Ⅲ) in Ferrihydrite'

机译：关于“直接观察水铁矿中四面体配位的Fe（Ⅲ）”的评论

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We have read with interest the discussion on recent work by Peak and Regier on the interpretation of the Fe L-edge spectrum of ferrihydrite. Having extensively studied Fe L-edge XAS spectra, we felt it important to point out some of the limitations in applying linear combinations to these types of spectra. In agreement with Manceau we do not believe that assignment of the presence or absence of tetrahedral sites in ferrihydrite is possible using linear combinations of L-edge spectra alone. However, our reasons for this conclusion are more general.

机译：我们感兴趣地阅读了Peak和Regier最近关于解释水铁矿Fe L边缘光谱的工作的讨论。在深入研究了Fe L边缘XAS光谱之后，我们感到重要的是指出在将线性组合应用于这些类型的光谱时的一些限制。与Manceau一致，我们认为仅使用L边缘光谱的线性组合就不可能确定三水铝石中四面体位置的存在或不存在。但是，我们得出此结论的原因更为笼统。

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《Environmental Science & Technology》 |2012年第20期|p.11471-11472|共2页
作者
Rosalie K. Hocking; Will P. Gates; John D. Cashion;
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作者单位

School of Pharmacy and Molecular Science, James Cook University, Townsville, QLD, 4811, Australia, and School of Chemistry, Monash University, Melbourne, Vic 3800, Australia;

Department of Civil Engineering, Monash University, Melbourne, Vic 3800, Australia, and SmecTech Research Consulting;

School of Physics, Monash University, Melbourne, Vic 3800, Australia;

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Comment on 'Direct Observation of Tetrahedrally Coordinated Fe(Ⅲ) in Ferrihydrite'

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