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Iodine Isotopes (~(129)I and ~(127)I) in the Baltic Proper, Kattegat and Skagerrak Basins

机译:波罗的海波普尔,卡特加特海峡和斯卡格拉克盆地的碘同位素(〜(129)I和〜(127)I)

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摘要

Radioactive anthropogenic pollution has raised concerns about the present and future environmental status of the semienclosed Baltic Sea. We here study the distribution and inventory of the anthropogenic radioactive ~(129)I in water depth profiles collected from 16 sites in August 2006 and 19 sites in April 2007 in the Baltic Proper and related Kattegat and Skagerrak basins. The results reveal considerable differences of ~(129)I concentration in terms of spatial and temporal variability and expose relatively high concentrations in the deep waters. Variability in the concentration of ~(127)I, stable natural isotope of iodine, seems to follow changes in the seawater salinity, but in oxygen-poor bottom waters sediment diagenetc release may contribute to the concentration of both isotopes in the water body. Inventory estimates show that ~(129)I in August 2006 (24.2 ± 15.4 kg) is higher than that in April 2007 (14.4 ± 8.3 kg) within the southern and central Baltic Proper whereas almost a constant load occurs in the Kattegat Basin. Calculated model inventory shows correspondence to empirical data and provides a guideline for future environmental assessment on the impact of ~(129)I load in the studied region.
机译:放射性人为污染已引起人们对半封闭波罗的海目前和未来环境状况的关注。我们在这里研究人为放射性〜(129)I在2006年8月从波罗的海珀尔及相关的Kattegat和Skagerrak盆地的16个站点和2007年4月的19个站点收集的水深剖面中的分布和清单。结果表明,就空间和时间变化而言,〜(129)I浓度存在相当大的差异,并且在深水中暴露出相对较高的浓度。稳定的碘自然同位素〜(127)I的浓度变化似乎随海水盐度的变化而变化,但是在氧气不足的底水中,沉积物的成岩等释放可能会导致水体中两种同位素的浓度升高。库存估算表明,波罗的海南部和中部地区2006年8月的〜(129)I(24.2±15.4 kg)高于2007年4月的(14.4±8.3 kg),而在Kattegat盆地几乎恒定地发生了负荷。计算得出的模型清单显示出与经验数据的对应关系,并为将来研究环境中〜(129)I负荷的影响提供了指南。

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  • 来源
    《Environmental Science & Technology》 |2011年第3期|p.903-909|共7页
  • 作者单位

    Department of Earth Sciences, Uppsala University, Uppsala, Sweden;

    rnDepartment of Earth Sciences, Uppsala University, Uppsala, Sweden,Dpartment of Geology, United Arab Emirates University, Al Ain, UAE;

    rnRiso National Laboratory for Sustainable Energy, Technical University of Denmark, Roskilde, Denmark;

    rnTandem Laboratory, Uppsala University Uppsala Sweden;

    rnRiso National Laboratory for Sustainable Energy, Technical University of Denmark, Roskilde, Denmark,Institute of Earth Environment, CAS, Xi'an 710075, China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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  • 正文语种 eng
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