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首页> 外文期刊>Environmental Science & Technology >Perfluorinated Compounds in Infiltrated River Rhine Water and Infiltrated Rainwater in Coastal Dunes
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Perfluorinated Compounds in Infiltrated River Rhine Water and Infiltrated Rainwater in Coastal Dunes

机译：沿海沙丘渗透的莱茵河水中和渗透雨水中的全氟化合物

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摘要

Different studies have shown that surface waters contain perfluorinated compounds (PFCs) in the low ng/L range. Surface waters are used to produce drinking water and PFCs have been shown to travel through the purification system and form a potentialthreatto human health. The specific physicochemical properties of PFCs cause them to be persistent and some of them to be bioaccumulative and toxic in the environment This study investigates the evolvement of PFC concentrations in Rhine water and rainwater during dune water infiltration processes over a transect in the dune area of the western part of The Netherlands. The difference between infiltrated river water and rainwater in terms of PFC composition was investigated. Furthermore, isomer profiles were investigated. The compound perfluorobutanesulfonate (PFBSI was found at the highest concentrations of all PFCs investigated, up to 37 ng/L in infiltrated river water (71 ± 13% of EPFCs). This is in contrast with the predominant occurrence of perfluorooctanoic acid (PFOA) and perfluorooctanesulfonate (PFOS) reported in literature. The concentrations of PFBS found in infiltrated river Rhine water were significantly higher than those in infiltrated rainwater. For perfluorohexanesulfonate (PFHxS)the opposite was found: infiltrated rainwater contained more than infiltrated river water. The concentrations of PFOA, perfluorohexanoic acid (PFHxA), perfluoroheptanoic acid (PFHpA), PFBS, PFOS, and PFHxS in infiltrated river water showed an increasing trend with decreasing age of the water. The relative contribution of the branched PFOA and PFOS isomers to total concentrations of PFOA and PFOS showed a decreasing trend with decreasing age of the water.
机译：不同的研究表明，地表水中的全氟化合物（PFC）含量低至ng / L。地表水用于生产饮用水，PFC已证明会通过净化系统，对人体健康构成潜在威胁。 PFC的特殊理化特性使其在环境中具有持久性，并且其中一些具有生物蓄积性和毒性。本研究调查了沙丘沙丘区某样地中沙丘水渗透过程中莱茵水和雨水中PFC浓度的变化。荷兰西部。研究了渗透河水和雨水在PFC成分方面的差异。此外，研究了异构体分布。全氟丁烷磺酸盐（PFBSI）在所有所研究的PFC中浓度最高，在渗透的河水中达到37 ng / L（占EPFC的71±13％），这与全氟辛酸（PFOA）和文献中报道了全氟辛烷磺酸盐（PFOS），在莱茵河入渗水中发现的PFBS浓度显着高于雨水入渗；相反，对于全氟己烷磺酸盐（PFHxS），则发现相反的情况：入渗雨水比入渗河水中含有更多的全氟辛烷磺酸。渗透河水中的全氟己酸（PFHxA），全氟庚酸（PFHpA），PFBS，PFOS和PFHxS随水龄的降低而呈增加趋势，支链PFOA和PFOS异构体对PFOA和PFOS总浓度的相对贡献全氟辛烷磺酸显示出随着水龄的减少而减少的趋势。

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  • 来源
    《Environmental Science & Technology》 |2010年第19期|p.7450-7455|共6页
  • 作者

    CHRISTIAN ESCHAUZIER; JORIS HAFTKA; PIETER J. STUYFZAND; PIM DE VOOGT;

  • 作者单位

    KWR Watercycte Research Institute, P.O.Box 1072, 3430 BB Nieuwegein, Netherlands Earth Surface Sciences, Institute for Biodiversity and Ecosystem Dynamics, Universiteit van Amsterdam, Science Park 904, 1098 XH Amsterdam, Netherlands;

    rnEarth Surface Sciences, Institute for Biodiversity and Ecosystem Dynamics, Universiteit van Amsterdam, Science Park 904, 1098 XH Amsterdam, Netherlands;

    rnKWR Watercycte Research Institute, P.O.Box 1072, 3430 BB Nieuwegein, Netherlands VU University Amsterdam, Faculty of Earth and Life Sciences, de Boelelaan 1085, 1081 HV Amsterdam, Netherlands;

    rnKWR Watercycte Research Institute, P.O.Box 1072, 3430 BB Nieuwegein, Netherlands Earth Surface Sciences, Institute for Biodiversity and Ecosystem Dynamics, Universiteit van Amsterdam, Science Park 904, 1098 XH Amsterdam, Netherlands;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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