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首页> 外文期刊>Environmental Science & Technology >Oxidation of Pharmaceuticals during Ozonation off Municipal Wastewater Effluents:A Pilot Study
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Oxidation of Pharmaceuticals during Ozonation off Municipal Wastewater Effluents:A Pilot Study

机译：臭氧在城市废水中臭氧氧化过程中的初步研究

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摘要

To reduce the release of Pharmaceuticals and endocrine disrupters into the aquatic environment or to remove them from wastewater intended for direct or indirect reuse,the application of advanced wastewater treatment may be required.In the present study,municipal wastewater effluents were treated with ozone (O_3) in a pilot-scale plant consisting of two bubble columns.The investigated effluents,which varied in suspended solids concentrations,comprised an effluent of conventional activated sludge treatment (CAS),the same effluent dosed with 15 mg of TSS L~(-1) of activated sludge (CAS + SS),and the effluent of a membrane bioreactor pilot plant (MBR).Selected classes of Pharmaceuticals were spiked in the wastewater at realistic levels ranging from 0.5 to 5 mug L~(-1).Samples taken at the inlet and the outlet of the pilot plant were analyzed with liquid chromatography (LC)-electrospray tandem mass spectrometry (MS).Macrolide and sulfonamide antibiotics,estrogens,and the acidic Pharmaceuticals diclofenac,naproxen,and indomethacin were oxidized by more than 90-99% for 0_3 doses >=2 mg L~(-1) in all effluents.X-ray contrast media and a few acidic Pharmaceuticals were only partly oxidized,but no significant differences were observed among the three effluents.These results show that many Pharmaceuticals present in wastewater can be efficiently oxidized with O_3 and that suspended solids have only a minor influence on the oxidation efficiency of nonsorbing micropollutants.
机译：为了减少药物和内分泌干扰物向水生环境中的释放或将其从拟直接或间接再利用的废水中去除，可能需要应用先进的废水处理方法。在本研究中，对市政废水进行了臭氧处理（O_3 ）在一个由两个鼓泡塔组成的中试规模的工厂中，所研究的废水随悬浮固体浓度的变化而变化，其中包含常规活性污泥处理（CAS）的废水，该废水的剂量为15 mg TSS L〜（-1） ）（活性污泥（CAS + SS））和膜生物反应器中试装置（MBR）的废水。选定类别的药物以0.5至5杯L〜（-1）的实际水平加标到废水中。用液相色谱（LC）-电喷雾串联质谱（MS）分析中试工厂的进样口和出样口.Macrolide和磺胺类抗生素，雌激素和酸性药物在所有废水中，0_3剂量> = 2 mg L〜（-1）时，als双氯芬酸，萘普生和消炎痛的氧化率均超过90-99％。X射线造影剂和一些酸性药物仅被部分氧化，但没有结果表明，三种废水之间存在显着差异。这些结果表明，废水中存在的许多药物都可以被O_3高效氧化，并且悬浮固体对非吸附性微污染物的氧化效率影响很小。

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  • 来源
    《Environmental Science & Technology》 |2005年第11期|p.4290-4299|共10页
  • 作者

    MARC M.HUBER; ANKE GOBEL; ADRIANO JOSS; NADINE HERMANN; DIRK LOFFLER; CHRISTA S.MCARDELL; ACHIM RIED; HANSRUEDI SIEGRIST; THOMAS A.TERNES; URS VON GUNTEN;

  • 作者单位

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

    Swiss Federal Institute for Environmental Science and Technology,Ueberlandstrasse 133,CH-8600 Duebendorf,Switzerland,Federal Institute of Hydrology,Am Mainzer Tor 1,D-56068 Koblenz,Germany,and WEDECO,Umwelttechnologie GmbH,Boschstrasse 6,D-32051 Herf;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 环境化学;
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