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Characterization of polycyclic aromatic hydrocarbons in PM2.5 and PM10 in Tanggu District, Tianjin Binhai New Area, China

机译:天津滨海新区塘沽区PM2.5 和PM10 中的多环芳烃特征

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摘要

Particulate matter (PM10 and PM2.5) concentrations were monitored during the November 2008 by using the filter samples collected day and night from three sites in Tanggu District at Tianjin Binhai New Area, China. The mean concentrations of PM2.5 and PM10 rank in the order of urban (150 μg/m3 for PM2.5 and 197 μg/m3 for PM10)industrial (32 μg/m3 for PM2.5 and 170 μg/m3 for PM10)suburb area (27 μg/m3 for PM2.5 and 59 μg/m3 for PM10). Sixteen polycyclic aromatic hydrocarbons (PAHs) were analyzed in PM10 and PM2.5 samples. Concentrations of total PAHs in PM2.5 and PM10 are in the range of 8.47–113.94 ng/m3 with average of 62.88 ng/m3 and 21.07–118.23 ng/m3 with average of 73.42 ng/m3, respectively. The light ring PAHs (2–4 rings) are dominant in both PM2.5 and PM10 during sampling time compares with the heavy ring (5–6 rings) PAHs. The relationship of PAHs and PM2.5 (r = 0.689, p0.05) is stronger than PAHs and PM10 (r = 0.570, p0.05), illustrating PAHs tend to adsorb in PM2.5. In addition, principal component analysis was applied to find the source of PAHs. Three principal factors representing three types of PAHs sources in Tanggu District are extracted, which were coke production, pyrogenic sources and vehicular source.
机译:使用从中国天津滨海新区塘沽区三个地点昼夜收集的过滤器样品,在2008年11月对颗粒物(PM10 和PM2.5 )的浓度进行了监测。 PM2.5 和PM10 的平均浓度按城市顺序排列(PM2.5 为150μg/ m3 ,197μg/ m3 PM10 )>工业(PM2.5 为32μg/ m3 ,PM10 )为170μg/ m3 )>郊区(27μg/ m3 < / sup>对于PM2.5 和59μg/ m3 对于PM10 )。在PM10 和PM2.5 样品中分析了16种多环芳烃(PAH)。 PM2.5 和PM10 中的总PAH浓度在8.47–113.94 ng / m3 范围内,平均为62.88 ng / m3 和21.07–118.23 ng / m3 m3 ,平均分别为73.42 ng / m3 。与重环(5-6个环)的PAH相比,在采样期间,轻环PAH(2-4个环)在PM2.5 和PM10 中均占主导地位。 PAHs与PM2.5 的关系(r = 0.689,p <0.05)优于PAHs和PM10 (r = 0.570,p <0.05),说明PAHs倾向于吸附在PM2.5中。此外,应用主成分分析来发现多环芳烃的来源。提取了代表塘沽区三种PAHs来源的三个主要因素,即焦炭产量,热源和车辆来源。

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  • 来源
    《Frontiers of Earth Science》 |2012年第3期|p.324-330|共7页
  • 作者单位

    State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan, 430074, China;

    State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan, 430074, China;

    State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan, 430074, China;

    State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan, 430074, China;

    Tianrenhe Researching and Developing Center of Environmental Protection Techniques, Tanggu, Tianjin, 300450, China;

    Tianrenhe Researching and Developing Center of Environmental Protection Techniques, Tanggu, Tianjin, 300450, China;

    Tianrenhe Researching and Developing Center of Environmental Protection Techniques, Tanggu, Tianjin, 300450, China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    PM2.5; PM10; polycyclic aromatic hydrocarbons (PAHs); Tanggu District; Tianjin Binhai New Area;

    机译:PM2.5;PM10;多环芳烃(PAHs);塘沽区;天津滨海新区;

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