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Hybrid catalyst of MoS2-CoMo2S4 on graphene for robust electrochemical hydrogen evolution

机译:MoS2-CoMo2S4在石墨烯上的杂化催化剂,用于稳健的电化学放氢

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摘要

After years of development, boosting the electrochemical hydrogen evolution performance of MoS2 catalyst through the traditional methods, such as defect engineering and conductivity improvement, has reached their limit. In this work, we propose a novel functional catalyst that is fabricated by hybrid two-dimensional nanostructures composed of MoS2 nanosheets and CoMo2S4 nanoplates in situ grown on graphene substrate for electrochemical hydrogen evolution reaction. The MoS2-CoMo2S4/graphene hybrid catalyst shows robust hydrogen evolution performance with low onset potential of 110 mV, high cathode current density of 85 mA cm(-2) at eta = 300 mV, and small Tafel slope of 42 mV dec(-1), as well as good durability. The excellent hydrogen evolution performance of the hybrid catalyst is likely attributed to the nonequilibrium composition, 2D structural advantages, conductive graphene substrate, and the electrocatalytic synergistic effect between MoS2 and CoMo2S4. (C) 2016 Elsevier Ltd. All rights reserved.
机译:经过多年的发展,通过缺陷工程和电导率改善等传统方法来提高MoS2催化剂的电化学制氢性能已达到极限。在这项工作中,我们提出了一种新颖的功能催化剂,该催化剂由在石墨烯衬底上原位生长的MoS2纳米片和CoMo2S4纳米片组成的二维二维混合结构制成,用于电化学制氢反应。 MoS2-CoMo2S4 /石墨烯杂化催化剂显示出强劲的氢释放性能,在eta = 300 mV时具有低的开始电势110 mV,高的阴极电流密度85 mA cm(-2)和小的Tafel斜率dec(-1) ),以及良好的耐久性。杂化催化剂出色的放氢性能可能归因于非平衡组成,二维结构优势,导电石墨烯基质以及MoS2和CoMo2S4之间的电催化协同效应。 (C)2016 Elsevier Ltd.保留所有权利。

著录项

  • 来源
    《Fuel》 |2016年第15期|559-564|共6页
  • 作者单位

    Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Key Lab Sci Anal Tumor Marker, Minist Educ, Qingdao 266042, Peoples R China;

    Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Key Lab Sci Anal Tumor Marker, Minist Educ, Qingdao 266042, Peoples R China;

    Agr Univ Hebei, Coll Sci & Technol, Cangzhou 061100, Peoples R China;

    Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Key Lab Sci Anal Tumor Marker, Minist Educ, Qingdao 266042, Peoples R China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Hydrogen evolution reaction; MoS2; CoMo2S4; Graphene; Energy conversion;

    机译:析氢反应;MoS2;CoMo2S4;石墨烯;能量转化;

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