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Femtosecond and Attosecond Spectroscopy in the XUV Regime

机译:XUV体制下的飞秒和阿秒光谱

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摘要

Attosecond-duration, fully coherent, extreme-ultraviolet (XUV) photon bursts obtained through laser high-harmonic generation have opened up new possibilities in the study of atomic and molecular dynamics. We discuss experiments elucidating some of the interesting energy redistribution mechanisms that follow the interaction of a high-energy photon with a molecule. The crucial role of synchronized, strong-field, near-IR laser pulses in XUV pump–probe spectroscopy is highlighted. We demonstrate that near-IR pulses can in fact be used to modify the atomic structure and control the electronic dynamics on attosecond timescales. Our measurements show that the Gouy phase slip in the interaction region plays a significant role in these attosecond experiments. We perform precision measurement of interferences between strong field-induced Floquet channels to extract the intensity and phase dependence of photoionization dynamics. Applications of emerging table-top ultrafast XUV sources in the study of core electron dynamics are also discussed.
机译:通过激光高次谐波产生获得的亚秒持续时间,完全相干的极紫外(XUV)光子爆发为原子和分子动力学研究开辟了新的可能性。我们讨论了阐明高能光子与分子相互作用后阐明的一些有趣的能量重新分配机制的实验。重点介绍了同步,强场,近红外激光脉冲在XUV泵浦光谱中的关键作用。我们证明了近红外脉冲实际上可以用来修改原子结构并控制阿秒级时标上的电子动力学。我们的测量结果表明,相互作用区域中的Gouy相滑在这些阿秒实验中起着重要作用。我们执行强场感应Floquet通道之间的干扰的精确测量,以提取光电离动力学的强度和相位依赖性。还讨论了新兴的台式超快XUV光源在核心电子动力学研究中的应用。

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