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首页> 外文期刊>Journal of Hazardous Materials >Polycyclic aromatic hydrocarbons at fire stations: firefighters' exposure monitoring and biomonitoring, and assessment of the contribution to total internal dose
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Polycyclic aromatic hydrocarbons at fire stations: firefighters' exposure monitoring and biomonitoring, and assessment of the contribution to total internal dose

机译：消防局的多环芳烃：消防员的暴露监测和生物监测，以及对内部总剂量贡献的评估

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摘要

This work characterizes levels of eighteen polycyclic aromatic hydrocarbons (PAHs) in the breathing air zone of firefighters during their regular work shift at eight Portuguese fire stations, and the firefighters' total internal dose by six urinary monohydroxyl metabolites (OH-PAHs). Total PAHs (Sigma PAHs) concentrations varied widely (46.4-428 ng/m(3)), mainly due to site specificity (urban/rural) and characteristics (age and layout) of buildings. Airborne PAHs with 2-3 rings were the most abundant (63.9-95.7% Sigma PAHs). Similarly, urinary 1-hydroxynaphthalene and 1-hydroxyacenaphthene were the predominant metabolites (66-96% Sigma OH-PAHs). Naphthalene contributed the most to carcinogenic Sigma PAHs (39.4-78.1%) in majority of firehouses; benzo[a]pyrene, the marker of carcinogenic PAHs, accounted with 1.5-10%. Statistically positive significant correlations (r >= 0.733, p <= 0.025) were observed between EPAHs and urinary Sigma OH-PAHs for firefighters of four fire stations suggesting that, at these sites, indoor air was their major exposure source of PAHs. Firefighter's personal exposure to PAHs at Portuguese fire stations were well below the existent occupational exposure limits. Also, the quantified concentrations of post-shift urinary 1-hydroxypyrene in all firefighters were clearly lower than the benchmark level (0:5 recommended by the American Conference of Governmental Industrial Hygienists. (C) 2016 Elsevier B.V. All rights reserved.
机译：这项工作的特点是，在葡萄牙八个消防局的常规工作期间，消防员的呼吸空气区域中有十八种多环芳香烃（PAHs）的水平，以及六种尿一羟基代谢物（OH-PAHs）对消防员的内部总剂量。总PAHs（Sigma PAHs）的浓度差异很大（46.4-428 ng / m（3）），主要归因于建筑物的场所特定性（城市/农村）和特征（年龄和布局）。带有2-3个环的机载PAH含量最高（63.9-95.7％Sigma PAH）。同样，尿中的1-羟基萘和1-羟基ac是主要的代谢产物（66-96％Sigma OH-PAHs）。在大多数消防站中，萘对致癌西格玛多环芳烃的贡献最大（39.4-78.1％）。致癌PAHs的标志物苯并[a] py占1.5-10％。在四个消防站的消防员中，EPAHs和尿Sigma OH-PAHs之间观察到统计学正相关（r> = 0.733，p <= 0.025），这表明在这些位置，室内空气是其主要暴露于PAHs。消防员在葡萄牙消防局对PAHs的个人暴露远低于现有的职业暴露极限。此外，所有消防员的班后尿1-羟基hydroxy的定量浓度明显低于基准水平（美国政府工业卫生专家会议建议的0：5。（C）2016 Elsevier B.V.保留所有权利。

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  • 来源
    《Journal of Hazardous Materials》 |2017年第ptaa期|184-194|共11页
  • 作者

    Oliveira Marta; Slezakova Klara; Alves Maria Jose; Fernandes Adilia; Teixeira Joao Paulo; Delerue-Matos Cristina; Pereira Maria do Carmo; Morais Simone;

  • 作者单位

    Inst Politen Porto, Inst Super Engn, REQUIMTE LAQV, R Dr Antonio Bernardino Almeida 431, P-4200072 Oporto, Portugal|Univ Porto, Fac Engn, Dept Engn Quim, LEPABE, R Dr Roberto Frias, P-4200465 Oporto, Portugal;

    Inst Politen Porto, Inst Super Engn, REQUIMTE LAQV, R Dr Antonio Bernardino Almeida 431, P-4200072 Oporto, Portugal|Univ Porto, Fac Engn, Dept Engn Quim, LEPABE, R Dr Roberto Frias, P-4200465 Oporto, Portugal;

    Escola Super Saude, Inst Politecn Braganca, Ave D Afonso 5, P-5300121 Braganca, Portugal;

    Escola Super Saude, Inst Politecn Braganca, Ave D Afonso 5, P-5300121 Braganca, Portugal;

    Inst Nacl Saude Publ, Dept Saude Ambiental, Rua Alexandre Herculano 321, P-4000055 Oporto, Portugal|Univ Porto, Inst Saude Publ, Rua Taipas 135, P-4050600 Oporto, Portugal;

    Inst Politen Porto, Inst Super Engn, REQUIMTE LAQV, R Dr Antonio Bernardino Almeida 431, P-4200072 Oporto, Portugal;

    Univ Porto, Fac Engn, Dept Engn Quim, LEPABE, R Dr Roberto Frias, P-4200465 Oporto, Portugal;

    Inst Politen Porto, Inst Super Engn, REQUIMTE LAQV, R Dr Antonio Bernardino Almeida 431, P-4200072 Oporto, Portugal;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Firefighters; Exposure; Polycyclic aromatic hydrocarbons (PAHs); Monohydroxyl-PAHs (OH-PAHs); 1-hydroxypyrene;

    机译：消防人员;暴露;多环芳烃（PAHs）;单羟基PAHs（OH-PAHs）;1-羟基py;

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