Thermodynamic equilibrium and kinetic fundamentals of oxide dissolution in aqueous solution

Jianwei Wang

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Thermodynamic equilibrium and kinetic fundamentals of oxide dissolution in aqueous solution

机译：水溶液中氧化物溶解的热力学平衡和动力学基础

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Dissolution of oxides in aqueous solutions is fundamentally important for a range of applications and a critical process that determines the chemical durability of industrial ceramics, the performance of nuclear waste forms, and the chemical weathering of minerals. The thermodynamic equilibrium and kinetics of dissolution reactions are key to determining the rate at which oxides dissolve. The increase in collaborative research across disciplines in materials research necessitates a common background to tackle shared scientific problems across different fields. This review selectively examines the fundamentals of dissolution theories that have been developed in chemistry, geochemistry, and materials science, and assembles them into a single collective document for the broader materials science community. Applications of the theories are highlighted using examples from specific areas, but can be similarly applied to other areas. Challenges and future research needs for a predictive-level understanding are discussed in light of the current literature.

机译：氧化物在水溶液中的溶解对于一系列应用以及确定工业陶瓷的化学耐久性，核废料形式的化学耐用性以及矿物质的化学风化的关键过程。溶解反应的热力学平衡和动力学是测定氧化物溶解的速率的关键。材料研究中的学科的协同研究的增加需要共同的背景来解决不同领域的共同科学问题。本综述选择性地研究了化学，地球化学和材料科学中开发的溶出理论的基础，并将其组织成为更广泛材料科学界的一个集体文件。使用特定区域的示例突出显示理论的应用，但可以类似地应用于其他区域。根据目前的文献讨论了预测层面理解的挑战和未来的研究需求。

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《Journal of Materials Research》 |2020年第8期|898-921|共24页
作者
Jianwei Wang;
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Department of Geology and Geophysics Center for Computation and Technology Louisiana State University Baton Rouge Louisiana 70803 USA;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
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正文语种 eng
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Thermodynamic equilibrium and kinetic fundamentals of oxide dissolution in aqueous solution

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