Co-mediated nucleation of erbium/silicon nanoclusters in fused silica

Mert Celikin; David Barba; Andreas Ruediger; Martin Chicoine; Francois Schiettekatte; Federico Rosei

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Co-mediated nucleation of erbium/silicon nanoclusters in fused silica

机译：熔融石英中/硅纳米团簇的共介导成核

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We investigate the structural evolution of Er/Si nanoclusters obtained in co-implanted fused silica upon annealing via Raman spectroscopy and transmission electron microscopy. The effect of annealing temperature (900-1200 ℃) on the nature and the relative fraction of the formed amorphous-Si, Si nanocrystals (Si-nc), and amorphous Er nanoparticles (Er-np) was determined in this ternary Er-Si-0 system, showing a change of growth regime above 1100 ℃ due to the formation of mixed Er/O/Si aggregates. We observe that the nucleation and growth of amorphous Er-np and Si-nc are mutually affected. The 2-fold increase in the size of Er-np when no excess Si~+ is present in the matrix indicates that the formation of Si-nc in the proximity of Er clusters hinders Er diffusivity above 1100 ℃. This finding shows the importance of nanoclustering for improving the thermal stability of Er-doped silica systems.

机译：我们调查了拉曼光谱和透射电子显微镜退火后共注入熔融石英中Er / Si纳米团簇的结构演变。在该三元Er-Si中测定了退火温度（900-1200℃）对所形成的非晶Si，Si纳米晶体（Si-nc）和非晶Er纳米颗粒（Er-np）的性质和相对分数的影响-0系统，由于混合的Er / O / Si聚集体的形成，在1100℃以上显示出生长方式的变化。我们观察到非晶Er-np和Si-nc的形核和生长相互影响。当基质中不存在过量的Si〜+时，Er-np的尺寸增加2倍，表明在1100℃以上Er团簇附近形成Si-nc阻碍了Er的扩散。该发现表明纳米簇对于改善掺Er的二氧化硅体系的热稳定性的重要性。

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《Journal of Materials Research》 |2015年第20期|3003-3010|共8页
作者
Mert Celikin; David Barba; Andreas Ruediger; Martin Chicoine; Francois Schiettekatte; Federico Rosei;
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Centre Energie Materiaux Telecommunications, Institut National de la Recherche Scientifique, Varennes, QC J3X 1S2, Canada;

Centre Energie Materiaux Telecommunications, Institut National de la Recherche Scientifique, Varennes, QC J3X 1S2, Canada;

Centre Energie Materiaux Telecommunications, Institut National de la Recherche Scientifique, Varennes, QC J3X 1S2, Canada;

Regroupement Quebecois sur les Materiaux de pointe, Departement de Physique, Universite de Montreal, Montreal, QC H3C 3J7, Canada;

Regroupement Quebecois sur les Materiaux de pointe, Departement de Physique, Universite de Montreal, Montreal, QC H3C 3J7, Canada;

Centre Energie Materiaux Telecommunications, Institut National de la Recherche Scientifique, Varennes, QC J3X 1S2, Canada and Center for Self-Assembled Chemical Structures, McGill University, Montreal, QC, H3A 0B8, Canada;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
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1. Silicon Nanocluster-sensitized Emission From Erbium: The Role Of Stress In The Formation Of Silicon Nanoclusters [J] . I. Ahmad, M. P. Temple, A. Kallis, Journal of Applied Physics . 2008,第12期

机译：Er引起的硅纳米簇致敏发射：应力在硅纳米簇形成中的作用
2. Formation of erbium-oxygen nanoclusters in erbium-doped oxidized amorphous silicon [J] . Bresler M, Gusev O, Terukov E, Physica status solidi, B. Basic research . 2005,第10期

机译：掺er氧化非晶硅中氧纳米团簇的形成
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机译：离子合成和离子掺杂方式对二氧化硅薄膜中硅纳米团簇对of发射的敏化作用的影响
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机译：掺silicon硅纳米团簇中的能量转移：富硅二氧化硅和硅纳米粉的比较
5. Towards an erbium-doped waveguide amplifier sensitized by silicon nanoclusters. [D] . Lenz, Florian C. 2009

机译：迈向由硅纳米团簇敏化的掺-波导放大器。
6. Evolution of the sensitized Er3+ emission by silicon nanoclusters and luminescence centers in silicon-rich silica [O] . Lingbo Xu, Dongsheng Li, Lu Jin, 2014

机译：富硅二氧化硅中硅纳米团簇和发光中心致敏的Er3 +发射的演化
7. Silicon nanocluster-sensitized emission from erbium: The role of stress in the formation of silicon nanoclusters [O] . Ahmad, I., Temple, M.P., Kallis, A., 2008

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8. Colloidal Au nanoclusters formed in fused silica by MeV ion implantation and annealing [R] . White, C. W., Zhou, D. S., Budai, J. D., 1993

机译：通过meV离子注入和退火在熔融二氧化硅中形成胶体au纳米团簇

Co-mediated nucleation of erbium/silicon nanoclusters in fused silica

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