Concurrent synthesis of methanol and methyl Formate catalyzed by copper-based catalysts II Influences of solvents and H_2/CO mole ratios

LIU Xing-Quan; WU Yu-Tang; LUO Shi-Zhong

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Concurrent synthesis of methanol and methyl Formate catalyzed by copper-based catalysts II Influences of solvents and H_2/CO mole ratios

机译：铜基催化剂同时催化合成甲醇和甲酸酯Ⅱ溶剂和H_2 / CO摩尔比的影响

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The concurrent synthesis of methanol and methyl formate (MF) form synthesis gas at low temperature and under low pressure in a slurry reactor has been investigated. The influences of the solvents and H_2/CO mole ratios on the activity and methyl formate selectivity of CuCl and Cu-Cr oxide catalysts have been examined. The experimental results demonstrate that the solvents have remarkable influences on the activity and methyl formate selectivity of CuCl and Cu-Cr oxide catalysts.

机译：已经研究了在淤浆反应器中在低温和低压下同时合成甲醇和甲酸甲酯（MF）形成合成气的方法。研究了溶剂和H_2 / CO摩尔比对CuCl和Cu-Cr氧化物催化剂的活性和甲酸甲酯选择性的影响。实验结果表明，溶剂对CuCl和Cu-Cr氧化物催化剂的活性和甲酸甲酯选择性有显着影响。

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来源
《Journal of Natural Gas Chemistry》 |1999年第3期|p.203-210|共8页
作者
LIU Xing-Quan; WU Yu-Tang; LUO Shi-Zhong;
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收录信息美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
原文格式 PDF
正文语种 eng
中图分类化学;
关键词
synthesis gas; methanol; methyl formate;

机译：合成气甲醇甲酸甲酯;

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专利

1. Concurrent synthesis of methanol and methyl Formate catalyzed by copper-based catalysts III. influence of concentrations of catalysts [J] . LIU Xing-Quan, CHEN Wen-kai, WU Yu-Tang Journal of Natural Gas Chemistry . 1999,第4期

机译：铜基催化剂同时催化合成甲醇和甲Format。催化剂浓度的影响
2. Concurrent synthesis of methanol and methyl Formate catalyzed by copper-based catalysts I. Influences of temperature and pressure [J] . LIU Xing-Quan, WU Yu-Tang, CHEN Wen-Kai Journal of Natural Gas Chemistry . 1999,第2期

机译：铜基催化剂同时催化合成甲醇和甲基甲酸酯I.温度和压力的影响
3. Hydrogenolysis of Methyl Formate by H_2/CO Mixtures with CuO/ZnO/Al_2O_3 Based Methanol Synthesis Catalysts [J] . G. Braca, A. M. Raspolli Galletti, N. J. Laniyonu, Industrial & Engineering Chemistry Research . 1995,第7期

机译：CuO / ZnO / Al_2O_3基甲醇合成催化剂通过H_2 / CO混合物加氢制甲酸甲酯
4. Hydrogenolysis of methyl formate to methanol on copper-based catalysts and TPR characterization [C] . Y. Long, W. Chu, Y. H. Ye, Natural Gas Conversion Symposium; 20040606-10; Dalian(CN) . 2004

机译：铜基催化剂上甲酸甲酯的氢解反应及TPR表征
5. I. Multicatalysis: Development of a Bismuth(III) triflate-catalyzed Nucleophilic addition/ Hydrofunctionalization Reaction in the Synthesis of Complex Heterocycles II. C--H Arylation of Arenes and Heteroarenes with Palladium-Carboxylate Catalysts: Identification of the Catalyst Resting State and the Crucial Role of Pivalate Ligand in Stabilization of the Catalyst III. C--H Arylation of Heteroarenes with Palladium-Carboxylate Catalysts: Importance of Phosphine Ligand for Basic Heteroarene Substrates IV. C--H Arylation of Heteroarenes with Palladium-Carboxylate Catalysts: Effect of the Properties of Basic Heteroarene Substrates on Direct Arylations. [D] . Tundel, Rachel E. 2011

机译：I.多催化作用：在复杂的杂环化合物的合成中三氟甲磺酸铋（III）催化的亲核加成/加氢官能化反应的发展。羰基钯催化剂对芳烃和杂芳烃的CH-H芳基化反应：催化剂静止状态的鉴定以及新戊酸酯配体在稳定催化剂中的关键作用III。羰基钯催化剂催化杂芳烃的CH芳基化：膦配体对基础杂芳烃基质的重要性IV。杂芳烃与钯-羧酸酯的CH芳基化：碱性杂芳烃底物性能对直接芳基化的影响。
6. Solvent Free Synthesis of PdZn/TiO2 Catalysts for the Hydrogenation of CO2 to Methanol [O] . Hasliza Bahruji, Jonathan Ruiz Esquius, Michael Bowker, -1

机译：无溶剂合成PdZn / TiO2催化剂用于将CO2加氢为甲醇
7. Tris (triphenylphosphine) rhodium(I) Chloride Catalyzed Synthesis of Methyl Formate from Methanol, Carbon Dioxide and Hydrogen in the Presence of a Tertiary Amine (Commemoration Issue Dedicated to Professor Eiichi Fujita on the Occasion of his Retirement) [O] . Phala Heng, Kudo Kiyoshi, Mori Sadayuki, 1985

机译：在叔胺存在下，由三（三苯基膦）氯化铑（I）催化由甲醇，二氧化碳和氢气合成甲基甲酸酯

Concurrent synthesis of methanol and methyl Formate catalyzed by copper-based catalysts II Influences of solvents and H_2/CO mole ratios

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