Platinum nanoparticles decorated robust binary transition metal nitride-carbon nanotubes hybrid as an efficient electrocatalyst for the methanol oxidation reaction

Zhan Guohe; Fu Zhenggao; Sun Dalei; Pan Zhanchang; Xiao Chumin; Wu Shoukun; Chen Chun; Hu Guanghui; Wei Zhigang

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Platinum nanoparticles decorated robust binary transition metal nitride-carbon nanotubes hybrid as an efficient electrocatalyst for the methanol oxidation reaction

机译：铂纳米颗粒装饰了坚固的二元过渡金属氮化物-碳纳米管杂化物，可作为甲醇氧化反应的高效电催化剂

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Titanium cobalt nitride (TiCoN)-CNTs hybrid support is prepared by a facile and efficient method, including a one-pot solvothermal process followed by a nitriding process, and this hybrid support is further decorated with Pt nanoparticles to catalyze the oxidation of methanol. The catalyst is characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS) and electrochemical measurements. Notably, Pt/CNTs@TiCoN catalyst exhibits a much higher mass activity and durability than that of the conventional Pt/C OM) for methanol oxidation. The experimental data indicates that the CNTs@TiCoN hybrid support combines the merits of the CNTs's high conductivity and the superb corrosion resistance of external TiCoN coating. (C) 2016 Elsevier B.V. All rights reserved.

机译：氮化钴钛（TiCoN）-CNTs杂化载体是通过一种简便而有效的方法制备的，包括一锅法溶剂热法和氮化法，然后将该杂化载体进一步用Pt纳米粒子修饰以催化甲醇的氧化。该催化剂通过X射线衍射（XRD），透射电子显微镜（TEM），X射线光电子能谱（XPS）和电化学测量来表征。值得注意的是，Pt / CNTs @ TiCoN催化剂显示出比常规Pt / C OM高得多的质量活性和耐久性，可用于甲醇氧化。实验数据表明，CNTs @ TiCoN杂化载体兼具CNTs高导电性和外部TiCoN涂层优异的耐腐蚀性的优点。（C）2016 Elsevier B.V.保留所有权利。

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来源
《Journal of power sources》 |2016年第15期|84-92|共9页
作者
Zhan Guohe; Fu Zhenggao; Sun Dalei; Pan Zhanchang; Xiao Chumin; Wu Shoukun; Chen Chun; Hu Guanghui; Wei Zhigang;
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作者单位

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

Huizhou King Brother Elect Technol Co Ltd, Huizhou 516083, Peoples R China;

Huizhou King Brother Elect Technol Co Ltd, Huizhou 516083, Peoples R China;

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

Guangdong Univ Technol, Sch Chem Engn & Light Ind, Guangzhou 510006, Guangdong, Peoples R China;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
原文格式 PDF
正文语种 eng
中图分类
关键词
Titanium cobalt nitride; Methanol oxidation reaction; Enhanced stability; Fuel cells;

机译：氮化钴钛甲醇氧化反应增强稳定性燃料电池;

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1. Platinum Nanoparticles Supported on Nitrobenzene-Functionalized Multiwalled Carbon Nanotube as Efficient Electrocatalysts for Methanol Oxidation Reaction [J] . Tao Li, Dou Shuo, Ma Zhaoling, Electrochimica Acta . 2015,第Null期

机译：硝基苯官能化多壁碳纳米管上负载的铂纳米颗粒作为甲醇氧化反应的高效电催化剂
2. Gold-platinum bimetallic nanotubes templated from tellurium nanowires as efficient electrocatalysts for methanol oxidation reaction [J] . Lu Chenchen, Kong Wei, Zhang Huying, Journal of power sources . 2015,第nova20期

机译：以碲纳米线为模板的金铂双金属纳米管作为甲醇氧化反应的有效电催化剂
3. Three-dimensional low-defect carbon nanotube/nitrogen-doped graphene hybrid aerogel-supported Pt nanoparticles as efficient electrocatalysts toward the methanol oxidation reaction [J] . Yan Minmin, Jiang Quanguo, Zhang Tao, Journal of Materials Chemistry, A. Materials for energy and sustainability . 2018,第37期

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4. Electrocatalysts for Ethanol and Methanol Oxidation Prepared by Ion Beam Assisted Deposition of Platinum and Rare Earths Metals on Carbon Fiber Paper Catalyst Carriers [C] . V. V. Poplavsky, A. V. Dorozhko, V. G. Matys Meeting of the Electrochemical Society . 2017

机译：通过离子束辅助沉积铂和稀土金属在碳纤维纸催化剂载体上制备的乙醇和甲醇氧化的电催化剂
5. Low Platinum-Group-Metal Electrocatalysts for Oxygen Reduction and Ammonia Oxidation Reactions [D] . Song, Liang . 2019

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6. Synthesis of transition metal sulfide and reduced graphene oxide hybrids as efficient electrocatalysts for oxygen evolution reactions [O] . Yu-Rim Hong, Sungwook Mhin, Jiseok Kwon, 2018

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8. Vertically Aligned BCN Nanotubes as Efficient Metal-Free Electrocatalysts for the Oxygen Reduction Reaction: A Synergetic Effect by Co- Doping with Boron and Nitrogen. [R] . Wang, S., Iyyamperumal, E., Roy, A., 2011

机译：垂直排列的BCN纳米管作为氧还原反应的高效无金属电催化剂：通过共掺杂硼和氮的协同效应。

Platinum nanoparticles decorated robust binary transition metal nitride-carbon nanotubes hybrid as an efficient electrocatalyst for the methanol oxidation reaction

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