Electrochemical modeling of single particle intercalation battery materials with different thermodynamics

Wei Lai

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Electrochemical modeling of single particle intercalation battery materials with different thermodynamics

机译：具有不同热力学的单粒子嵌入电池材料的电化学建模

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Current-voltage relations of a single intercalation battery electrode particle were modeled with the step current, step voltage, linear sweep voltage, and sinusoidal current signals. A solid solution with constant diffusivity, a solid solution with variable diffusivity, and a phase transformation material were considered for their thermodynamic and kinetic evaluations based on the regular solution model and the generalized Poisson-Nernst-Planck equations. The numerical simulation results were compared with known, small-signal solutions and experimental data throughout the article.

机译：使用阶跃电流，阶跃电压，线性扫描电压和正弦电流信号对单个插入式电池电极颗粒的电流-电压关系进行建模。基于规则溶液模型和广义Poisson-Nernst-Planck方程，考虑了具有恒定扩散率的固溶体，具有可变扩散率的固溶体和相变材料的热力学和动力学评估。在整个文章中，将数值模拟结果与已知的小信号解决方案和实验数据进行了比较。

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来源
《Journal of power sources》 |2011年第15期|p.6534-6553|共20页
作者
Wei Lai;
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作者单位

Department of Chemical Engineering and Materials Science, Michigan State University, East Lansing, Ml 48824, USA;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
原文格式 PDF
正文语种 eng
中图分类
关键词
single particle; intercalation battery; regular solution; phase transformation; poisson-nernst-planck; current-voltage relation;

机译：单颗粒插层电池;定期解决;相变泊松内斯特-普朗克电流电压关系;

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Electrochemical modeling of single particle intercalation battery materials with different thermodynamics

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