Development of tellurium-modified carbon catalysts for oxygen reduction reaction in PEM fuel cells

Xuguang Li; Lingyun Liu; Jong-Won Lee; Branko N. Popov

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Development of tellurium-modified carbon catalysts for oxygen reduction reaction in PEM fuel cells

机译：用于PEM燃料电池中氧还原反应的碲改性碳催化剂的开发

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Tellurium (Te)-modified carbon catalyst for oxygen reduction reaction was prepared through chemical reduction of telluric acid followed by the pyrolysis process at elevated temperatures. The catalyst was found to be active for oxygen reduction reaction. High-temperature pyrolysis plays a crucial role in the formation of the active sites of the catalysts. When the pyrolysis was conducted at 1000℃, the catalyst exhibited the onset potential for oxygen reduction as high as 0.78 V vs. NHE and generated less than 1% H_2O_2 during oxygen reduction. The performance of the membrane-electrode assembly prepared with the Te-modified carbon catalyst was also evaluated.

机译：通过将碲酸化学还原，然后在高温下进行热解过程，制备了用于氧还原反应的碲（Te）改性碳催化剂。发现该催化剂对氧还原反应具有活性。高温热解在催化剂活性部位的形成中起关键作用。当在1000℃进行热解时，该催化剂表现出的氧还原起始电位相对于NHE高达0.78 V，并且在氧还原过程中生成的H_2O_2小于1％。还评估了用Te-改性的碳催化剂制备的膜-电极组件的性能。

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来源
《Journal of power sources》 |2008年第1期|p.18-23|共6页
作者
Xuguang Li; Lingyun Liu; Jong-Won Lee; Branko N. Popov;
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作者单位

Center for Electrochemical Engineering, Department of Chemical Engineering, University of South Carolina, Columbia, SC 29208, USA;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
原文格式 PDF
正文语种 eng
中图分类能源与动力工程;
关键词
tellurium; carbon catalyst; oxygen reduction; polymer electrolyte membrane fuel cell;

机译：碲;碳催化剂;氧还原;聚合物电解质膜燃料电池;

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专利

1. Development Of High Performance Carbon Composite Catalyst For Oxygen Reduction Reaction In Pem Proton Exchange Membrane Fuel Cells [J] . Vijayadurga Nallathambi, Jong-Won Lee, Swaminatha P. Kumaraguru, Journal of power sources . 2008,第1期

机译：Pem质子交换膜燃料电池氧还原反应用高性能碳复合催化剂的研制
2. Studies of oxygen reduction reaction active sites and stability of nitrogen-modified carbon composite catalysts for PEM fuel cells [J] . Gang Liu, Xuguang Li, Prabhu Ganesan, Electrochimica Acta . 2010,第8期

机译：氧还原反应活性位点及氮素改性碳复合催化剂稳定性的PEM燃料电池
3. Development of non-precious metal oxygen-reduction catalysts for PEM fuel cells based on N-doped ordered porous carbon [J] . Gang Liu, Xuguang Li, Prabhu Ganesan Applied Catalysis, B. Environmental: An International Journal Devoted to Catalytic Science and Its Applications . 2009,第1a2期

机译：基于N掺杂有序多孔碳的PEM燃料电池非贵金属氧还原催化剂的开发
4. Development of Nitrogen-Modified Carbon-Based Catalysts for Oxygen Reduction in PEM Fuel Cells [C] . Vijayadurga Nallathambi, Xuguang Li, Jong-Won Lee, Proton Exchange Membrane Fuel Cells 8 . 2008

机译：用于PEM燃料电池中氧还原的氮改性碳基催化剂的开发
5. Development of platinum-free electrocatalysts for oxygen reduction reaction in the PEM fuel cell. [D] . Liu, Lingyun. 2006

机译：开发用于PEM燃料电池中氧还原反应的无铂电催化剂。
6. Metal–Organic‐Framework‐Derived Dual Metal‐ and Nitrogen‐Doped Carbon as Efficient and Robust Oxygen Reduction Reaction Catalysts for Microbial Fuel Cells [O] . Haolin Tang, Shichang Cai, Shilei Xie, 2016

机译：金属-有机框架衍生的双金属和氮掺杂碳可作为微生物燃料电池的高效稳健的氧还原反应催化剂
7. A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: nanostructure, activity, mechanism and carbon support in PEM fuel cells [O] . Sui, Sheng, Wang, Xiaoying, Zhou, Xintong, 2017

机译：用于氧还原反应的Pt电催化剂的全面综述：PEM燃料电池中的纳米结构，活性，机理和碳载体

Development of tellurium-modified carbon catalysts for oxygen reduction reaction in PEM fuel cells

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