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Spin fluctuations in YBa_2Cu_3O_(6.6)

机译:YBa_2Cu_3O_(6.6)中的自旋涨落

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An important feature of the high-transition-temperature (high-T_c) copper oxide superconductors is the magnetism that results from the spins associated with the incomplete outer electronic shells (3d~9) of the copper ions. Fluctuations of these spins give rise to magnetic excitations of the material, and might mediate the electron pairing that leads to superconductivity. If the mechanism for high-T_c superconductivity is the same for all copper oxide systems, their spin fluctuations should be universal. But so far, the opposite has seemed to be the case: neutron scattering data reveal clear differences between the spin fluctuations for two major classes of high- T_c materials, La_(2-x)Sr_xCuO_4 (refs 1-3) and YBa_2Cu_3O_(7-x) (refs 4-6), whose respective building blocks are CuO_2 layers and bilayers. Here we report two-dimensional neutron-scattering imaging of YBa_2Cu_3O_(6.6), which reveals that the low-frequency magnetic excitations are virtually identical to those of similarly doped La_(2-x)Sr_xCuO_4. Thus, the high-temperature (T_c approx< 92 K) superconductivity of the former materials may be related to spatially coherent low-frequency spin excitations that were previously thought to be unique to the lower- T_c (< 40 K) single-layer La_(2-x)Sr_xCuO_4 family.
机译:高转变温度(high-T_c)氧化铜超导体的一个重要特征是磁性,该磁性是由与铜离子不完整的外部电子外壳(3d〜9)相关的自旋所产生的。这些自旋的波动会引起材料的磁激发,并可能介导导致超导的电子对。如果对于所有氧化铜系统来说,高T_c超导性的机理都相同,则它们的自旋涨落应该是普遍的。但到目前为止,情况似乎恰恰相反:中子散射数据揭示出两种主要的高T_c材料La_(2-x)Sr_xCuO_4(参考1-3)和YBa_2Cu_3O_(7)的自旋涨落之间存在明显差异。 -x)(参考文献4-6),其各自的构成模块是CuO_2层和双层。在这里,我们报告YBa_2Cu_3O_(6.6)的二维中子散射成像,它揭示了低频磁激发实际上与相似掺杂的La_(2-x)Sr_xCuO_4的激发相同。因此,前一种材料的高温(T_c约<92 K)超导性可能与空间相干的低频自旋激发有关,以前人们认为它们是较低的T_c(<40 K)单层La_唯一的。 (2-x)Sr_xCuO_4系列。

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