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Anti-Stokes fluorescence of Cr~(3+) ions doped crystals excited in one-phonon vibronic sidebands

机译:一声子振动子边带中激发的Cr〜(3+)离子掺杂晶体的反斯托克斯荧光

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摘要

The fluorescence of Cr3+ ions doped insulating crystals was studied under the laser excitation within the one-phonon vibronic sidebands of zero-phonon (4)A(2) - E-2 transitions. The phonon-assisted anti-Stokes fluorescence spectra were observed at ambient and liquid nitrogen temperature. The spectroscopic results suggest that one-phonon vibronic sidebands of zero-phonon lines in impurity ions fluorescence spectra are of interest from the point of view of achieving optical refrigeration starting at ambient temperature as well as significantly below it.
机译:在零声子(4)A(2)-E-2跃迁的单声子振动边带内的激光激发下研究了Cr3 +离子掺杂的绝缘晶体的荧光。在环境温度和液氮温度下观察到了声子辅助的反斯托克斯荧光光谱。光谱结果表明,从实现从环境温度开始以及显着低于环境温度的光学制冷的观点来看,杂质离子荧光光谱中零声子线的单声子振动边带是令人关注的。

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