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Enhanced and tunable nonlinear optical responses of nitrogen-doped nickel oxide induced by femtosecond laser excitation

机译:由飞秒激光激发诱导的氮掺杂氧化镍的增强和可调谐非线性光学响应

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摘要

In this work, we report the impact of nitrogen (N) doping in nickel oxide films on nonlinear optical responses (NORs) utilizing 532 nm, 330 fs laser pulses with both linear and radial polarization states. The pristine and N-doped NiO films are grown through radio frequency magnetron sputtering technique and further characterized by AFM, UV-Vis transmittance spectra and XP S. The experimental results demonstrate that NORs, including reverse saturable absorption and optical Kerr refraction, of the as-prepared NiO films along with their optical power limiting (OPL) are intimately related to the N doping and the laser polarization patterns. More specifically, both the NORs and OPL increase scalingly with the doping concentration under the linearly polarized laser excitation. The strongest optical nonlinear absorption coefficient, optical nonlinear refraction index and OPL efficiency are in turn determined to be 4.55 x 10(-7) m/W, 6.5 x 10(-16) m(2)/W and 50% for the heaviest N-implanted NiO film. In a sharp contrast, for the raidally polarized beam impinging onto the pristine and doped NiO films, the NORs and OPL initially drop off and then strengthen together as the increases of N-implanted content. Such enhanced and tunable NORs are due to the fact that the involvement of doping state gives rise to promoted optical transitions originating from the narrowing of band gap, as well as the use of ultrafast vectorial laser induces anisotropic nonlinearity and intricate light-matter interplay. Our results will open a new perspective to develop optical power limiter and ultrafast photonic devices.
机译:在这项工作中,我们报告了利用532nm,330 fs激光脉冲与线性和径向偏振态的非线性光学响应(nOR)对非线性光学响应(nors)的氮气(n)掺杂的影响。原始和N掺杂的NiO膜通过射频磁控溅射技术生长,并且通过AFM,UV-VIS透射谱和XP S的进一步表征。实验结果表明,包括反向可饱和的吸收和光学克尔折射,如 - 与它们的光学电源限制(OPL)一起进行制备的NIO薄膜与N掺杂和激光偏振图案密切相关。更具体地,NOR和OPL均匀地随着线性偏振激光激发下的掺杂浓度而增加。最强的光学非线性吸收系数,光学非线性折射指数和OPL效率又确定为4.55×10(-7)m / w,6.5×10(-16)m(2)/ w,最重50% N-植入的NiO膜。在一个鲜明的对比中,对于撞击原始和掺杂的NiO膜的raidizally偏振射线,NOR和OPL最初脱落,然后加强在一起,随着N-植入含量的增加。这种增强和可调谐的内心是由于掺杂状态的参与导致源自带隙缩小的促进光学转变,以及超快vrsial激光诱导各向异性非线性和错综复杂的浅品相互作用。我们的结果将开创新的视角,以开发光学电源限制器和超快光子器件。

著录项

  • 来源
    《Optical Materials》 |2020年第8期|109987.1-109987.9|共9页
  • 作者单位

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

    Taiyuan Univ Technol Coll Phys & Optoelect Key Lab Adv Transducers & Intelligent Control Sys Minist Educ & Shanxi Prov Taiyuan 030024 Peoples R China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Nickel oxide; Third-order optical nonlinearity; Magnetron sputtering technique; Radially polarized beam; Optical power limiting;

    机译:氧化镍;三阶光学非线性;磁控溅射技术;径向偏振光梁;光功率限制;

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