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Observation of strong exciton--photon coupling in semiconductor microcavities containing organic dyes and J-aggregates

机译:含有有机染料和J聚集体的半导体微腔中强激子-光子耦合的观察

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We report the observation of the strong-coupling regime between organic excitons and confined photons within a microcavity structure. As the optically active organic semiconductors within our devices, we have used the organic dye tetra-(2,6-tert-butyl)phenolpor zinc [4TBPPZn] which has an intense narrow "Soret" band absorption and also a cyanine dye which can form so-called "J-aggregates". Strong exciton--photon coupling is demonstrated from the anti- crossing of exciton and photon modes. Room temperature vacuum-Rabi splittings more than one order of magnitude larger than the highest values reported for inorganic semiconductors are observed. Such results open the way to structures in which new hybrid states of organic and inorganic excitons can be expected.
机译:我们报告了在微腔结构内有机激子和受限光子之间的强耦合机制的观察。作为我们设备中的光学活性有机半导体,我们使用了有机染料四-(2,6-叔丁基)苯酚锌[4TBPPZn],该锌具有很强的“ Soret”窄带吸收能力,并且还可以使用花青染料所谓的“ J聚合”。激子和光子模式的反交叉证明了强激子-光子耦合。观察到室温真空-拉比裂解比无机半导体报道的最高值大一个数量级。这样的结果为可以期待有机和无机激子的新混合态的结构开辟了道路。

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