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Some optical properties of Cr~4+-doped crystals

机译:Cr〜4 +掺杂晶体的某些光学性质

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We summarize briefly some of our past studies, and report of preliminary recent new results concerning the optical properties of Cr~4+-doped crystals that are important for utilization as passive Q-switching devices in NdtYAG 1aser systems. The host crystals involved are YAG, YSGG, GGG, LuAG and forsterite. Excited-state lifetimes of 4.0, l.0 and 1.7 μs were measured by the Cr~4+ fluorescence decay (l.3--l.7 μm) following pulsed excitation at l064 nm in YAG, YSGG and GGG, respectively. The ground- and excited-state absorption (ESA) cross-sections at λ = l064 nm were estimated from transmission saturation measurements. For [Cr~4+Mg~2+]:YAG the respective results were σgs = (3.25 ± 0.15) x l0~-18 cm~2 and σes = (6.25 ± 0.5) x l0~-l9 cm~2. In the orthorhombic forsterite, the cross-sections were polar- ization dependent. We got ags < (3.3 ± l) x l0~-l9 cm~2 for EⅡa, σgs = (23 ± 2) x l0~-l9 cm~2 and σes = (9.0 ± 0.7) x l0~-l9 cm~2 for EⅡb, and σgs = (16 ± l) x l0~-l9 cm~2 and σes = (5.7 ± 0.4) x l0~-l9 cm~2 for EⅡc. Polarised ESA spectra were measured between 680 and 960 nm using the pulsed pump/probe technique. At 750 nm we got σgs = (110 ± l0) x l0~-19 cm~2 and σes = (25 ± 3) x 10~-l9 cm~2 for EⅡb. Passive Q-switching performance of a flashlamp-pumped Nd:YAG laser using an intracavity [Cr~4+,Ca~2+]:GGG sample is also demonstrated.
机译:我们简要总结了我们过去的一些研究,并报告了有关Cr〜4 +掺杂晶体的光学性质的最新近期初步结果,这些结果对于在NdtYAG 1aser系统中用作无源Q开关器件很重要。涉及的主体晶体是YAG,YSGG,GGG,LuAG和镁橄榄石。在YAG,YSGG和GGG中分别在1064 nm处进行脉冲激发后,Cr〜4 +荧光衰减(1.3--1.7μm)测得的激发态寿命为4.0、1.0和1.7μs。 λ= 1064 nm处的基态和激发态吸收(ESA)截面是根据透射饱和度测量值估算的。对于[Cr〜4 + Mg〜2 +]:YAG,各自的结果为σgs=(3.25±0.15)x l0〜-18 cm〜2和σes=(6.25±0.5)x l0〜-19 cm〜2。在斜方镁橄榄岩中,横截面与极化有关。 EⅡa的ags <(3.3±l)x l0〜-9 cm〜2,σgs=(23±2)x l0〜-l9 cm〜2和σes=(9.0±0.7)x l0〜-9 cm〜 EⅡb为2,σgs=(16±l)x l0〜-19 cm〜2,σes=(5.7±0.4)x l0〜-9 cm〜2。使用脉冲泵浦/探针技术在680至960 nm之间测量了极化ESA光谱。在750 nm处,EⅡb的σgs=(110±10)x l0〜-19 cm〜2,σes=(25±3)x 10〜-19 cm〜2。还证明了使用腔内[Cr〜4 +,Ca〜2 +]:GGG样品的闪光灯泵浦Nd:YAG激光器的无源Q开关性能。

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