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Erratum: State-selective intersystem crossing in nitrogen-vacancy

机译：勘误表：氮空位的状态选择系统间穿越

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We have become aware that the vibrational overlap function F(A), which is defined in Eq. (5), was incorrectly normalized. This quantity factors into the intersystem crossing (ISC) rates Γ_(At), and Γ_(E_(1,2)) from the states |A_1> and |E_(1,2)> [Eqs. (6) and (13), respectively]. As a result, the theoretical value of Γ_(A1) that is plotted in Fig. 5 is too large by a factor of 2π. We thank A. Gali for bringing this error to our attention. We have also reexamined an assumption regarding the transverse spin-orbit coupling rate λ_⊥ and found it not to be valid. The dynamic Jahn-Teller effect in the ~3E excited state manifold causes the strengths of the spin-orbit interaction and the excited states' response to externally applied fields to be reduced [1] by a quantity known as the Ham reduction factor [2]. This factor changes the value of λ_⊥ that also enters into both intersystem crossing (ISC) rates. We had previously assumed that this effect is negligible, but we discovered this not to be the case when we explicitly calculated the Ham reduction factor. The magnitude of this effect for the NV center and its implications for the ISC are topics of current theoretical interest, so we present our explicit calculation of the Ham reduction factor here.
机译：我们已经意识到，振动重叠函数F（A）在等式中定义。 （5），被错误归一化。此数量从状态| A_1>和| E_（1,2）> [等式]分解为系统间交叉（ISC）比率Γ_（At）和Γ_（E_（1,2））。 （6）和（13）]。结果，图5中绘制的Γ_（A1）的理论值太大了2π。我们感谢A. Gali提请我们注意此错误。我们还重新检查了关于横向自旋轨道耦合率λ_⊥的假设，并发现该假设无效。 〜3E激发态流形中的动态Jahn-Teller效应使自旋轨道相互作用的强度和激发态对外部施加场的响应降低[1]，减少量称为Ham降低因子[2]。 。该因子改变了λ_⊥的值，该值也同时进入两个系统间交叉（ISC）速率。以前我们假设这种影响可以忽略不计，但是当我们明确计算Ham降低因子时，发现情况并非如此。对NV中心的这种影响的大小及其对ISC的影响是当前理论上感兴趣的主题，因此，在此我们对Ham降低因子进行显式计算。

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