Equilibrium free energy measurement of a confined electron driven out of equilibrium

A. Hofmann; V. F. Maisi; C. Roessler; J. Basset; T. Kraehenmann; P. Maerki; T. Ihn; K. Ensslin; C. Reichl; W. Wegscheider

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Equilibrium free energy measurement of a confined electron driven out of equilibrium

机译：失去平衡的受限电子的平衡自由能测量

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The Jarzynski equality relates nonequilibrium thermodynamics and equilibrium states. We realize a coupled quantum dot-electron reservoir system in which the time resolved observation of the tunneling dynamics is used to explicitly measure the exerted work and dissipated heat per single charge. We determine accurate values of the equilibrium free energy change over a large range of final state energies by driving the system far from equilibrium.

机译：Jarzynski等式涉及非平衡热力学和平衡状态。我们实现了一个耦合的量子点电子储层系统，其中对隧道动力学的时间分辨观察被用于显式测量每单电荷的功和耗散热。通过驱动系统远离平衡状态，我们确定了在较大范围的最终状态能量范围内的平衡自由能变化的准确值。

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《Physical review》 |2016年第3期|035425.1-035425.5|共5页
作者
A. Hofmann; V. F. Maisi; C. Roessler; J. Basset; T. Kraehenmann; P. Maerki; T. Ihn; K. Ensslin; C. Reichl; W. Wegscheider;
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Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

Solid State Physics Laboratory, ETH Zuerich, 8093 Zuerich, Switzerland;

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1. Equilibrium free energy measurement of a confined electron driven out of equilibrium [J] . Hofmann A., Maisi V. F., Roessler C., Physical review, B . 2016,第3期

机译：失去平衡的受限电子的平衡自由能测量
2. Near-Equilibrium Measurements of Nonequilibrium Free Energy [J] . David A. Sivak, Gavin E. Crooks Physical review letters . 2012,第15期

机译：非平衡自由能的近平衡测量
3. Determination of equilibrium free energy from nonequilibrium work measurements [J] . L. Y. Chen, D. A. Bastien, H. E. Espejel Physical chemistry chemical physics: PCCP . 2010,第25期

机译：从非纤维工作测量中测定平衡的自由能
4. Direct measurement of single molecular interaction free energies at solid/liquid interfaces based on non-equilibrium force spectroscopy [C] . Thomas Utzig, Sangeetha Raman, Philipp Stock, World biomaterials congress . 2016

机译：基于非平衡力谱直接测量固/液界面上单分子相互作用的自由能
5. Imaging of metallic multilayer structures through nonequilibrium electron transport and energy dynamics of nonequilibrium electrons in thin aluminum films. [D] . Guerra, Arnold, III. 1999

机译：通过非平衡电子传输和铝薄膜中非平衡电子的能量动力学对金属多层结构进行成像。
6. From the Cover: Bias and error in estimates of equilibrium free-energy differences from nonequilibrium measurements [O] . Jeff Gore, Felix Ritort, Carlos Bustamante 2003

机译：从封面开始：来自非平衡测量的平衡自由能差异估计中的偏差和误差
7. Equilibrium free energy measurement of a confined electron driven out of equilibrium [O] . Hofmann, Andrea, Maisi, Ville F., Rössler, Clemens, 2015

机译：受限制电子驱动的平衡自由能测量平衡

Equilibrium free energy measurement of a confined electron driven out of equilibrium

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