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Quantification of the magnetic exchange via element-selective high-field magnetometry: Co-doped ZnO epitaxial films

机译:通过元素选择性高场磁力分析法对磁交换进行定量:共掺杂ZnO外延膜

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摘要

We have measured the element specific M(H) curves for 5%, 10%, and 15% Co-doped ZnO epitaxial films with high crystalline perfection using x-ray magnetic circular dichroism (XMCD). The XMCD(H) curves do not saturate up to 17 T directly evidencing antiferromagnetic exchange between neighboring Co dopant atoms. Angular-dependent XMCD(H) measurements in combination with theoretical calculations based on a well-established model Hamiltonian allow to determine both the next-neighbor exchange J as well as the single ion anisotropy D quantitatively. While for 5% and 10% Co doping, J = 15 K and D = 3K, for 15% Co doping, they are reduced to 10 and 2 K, respectively. High-field, element selective magnetometry based on XMCD is thus shown to be a suitable technique to determine microscopic magnetic parameters even in thin epitaxial films of dilute magnetic systems.
机译:我们已经使用X射线磁圆二向色性(XMCD)测量了5%,10%和15%的Co掺杂的ZnO外延膜的元素比M(H)曲线,具有高的晶体完美度。 XMCD(H)曲线不饱和到17 T,直接表明相邻Co掺杂原子之间的反铁磁交换。角度相关的XMCD(H)测量与基于完善模型哈密顿量的理论计算相结合,可以定量确定下一个邻域交换J和单个离子各向异性D。对于5%和10%的Co掺杂,J = 15 K和D = 3K,对于15%的Co掺杂,它们分别减小到10和2K。因此,即使在稀磁系统的外延薄膜中,基于XMCD的高场元素选择性磁法也被证明是一种确定微观磁参数的合适技术。

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  • 来源
    《Physical review》 |2012年第24期|p.245202.1-245202.8|共8页
  • 作者单位

    Fakultaet fuer Physik, Universitaet Duisburg-Essen, Lotharstr. 1, D-47057 Duisburg, Germany,Institut fur Halbleiter- und Festkoerperphysik, Johannes Kepler Universitaet, A-4040 Linz, Austria;

    Fakultaet fuer Physik, Universitaet Duisburg-Essen, Lotharstr. 1, D-47057 Duisburg, Germany,Institut fur Halbleiter- und Festkoerperphysik, Johannes Kepler Universitaet, A-4040 Linz, Austria;

    European Synchrotron Radiation Facility (ESRF), 6 Rue Jules Horowitz, BP 220, 38043 Grenoble Cedex, France;

    European Synchrotron Radiation Facility (ESRF), 6 Rue Jules Horowitz, BP 220, 38043 Grenoble Cedex, France;

    Fakultaet fuer Physik, Universitaet Duisburg-Essen, Lotharstr. 1, D-47057 Duisburg, Germany;

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  • 正文语种 eng
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  • 关键词

    X-ray absorption spectra; crystal-field theory and spin hamiltonians; magnetic properties of monolayers and thin films;

    机译:X射线吸收光谱;晶体场理论和自旋哈密顿论;单层和薄膜的磁性;

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