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首页> 外文期刊>Physical review >Far-infrared optical study of electromagnons and their coupling to optical phonons in Eu_(1-x)Y_xMnO_3 (x=0.1, 0.2, 0.3, 0.4, and 0.45)
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Far-infrared optical study of electromagnons and their coupling to optical phonons in Eu_(1-x)Y_xMnO_3 (x=0.1, 0.2, 0.3, 0.4, and 0.45)

机译:Eu_(1-x)Y_xMnO_3(x = 0.1、0.2、0.3、0.4和0.45)中电磁子及其与声子耦合的远红外光学研究

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摘要

A systematic far-infrared optical study has been performed on multiferroic oxides Eu_(1-x)Y_xMnO_3 (x=0.1, 0.2, 0.3, 0.4, and 0.45) in which versatile characteristics of magnetic orders including the ab- and bc-plane spiral, A-type antiferromagnetic, and collinear sinusoidal states show up, depending on Y content (x) and temperature. We have observed evolution of various absorption bands below 100 cm~(-1), which critically depends on the nature of magnetic order and hence can be assigned to magnetic excitations. The spiral-spin structures yield the most intense absorption composed of two pronounced peak structures around 20 and 65 cm~(-1), while the spectra for the collinear sinusoidal spin structure exhibit a plateaulike shape below 80 cm~(-1). In contrast, the A-type antiferromagnetic phase shows no electrically active spin excitation. A quantitative analysis shows their strong mutual coupling in the spiral-spin phases as manifested by the transfer of the spectral weight between the electrically active spin excitations and the lowest optical-phonon mode.
机译:已对多铁氧化物Eu_(1-x)Y_xMnO_3(x = 0.1、0.2、0.3、0.4和0.45)进行了系统的远红外光学研究,其中包括ab平面和bc平面螺旋的磁阶的通用特性,取决于Y含量(x)和温度,出现A型反铁磁和共线正弦波状态。我们已经观察到低于100 cm〜(-1)的各种吸收带的演化,这主要取决于磁阶的性质,因此可以归因于磁激发。螺旋自旋结构产生最强烈的吸收,该吸收由在20和65 cm〜(-1)附近的两个明显的峰结构组成,而共线正弦自旋结构的光谱在80 cm〜(-1)以下表现出高原样的形状。相反,A型反铁磁相未显示出电活性自旋激发。定量分析显示了它们在螺旋自旋相中的强相互耦合,这通过电活性自旋激发与最低光学声子模式之间的频谱权重转移得以体现。

著录项

  • 来源
    《Physical review》 |2009年第21期|214431.1-214431.8|共8页
  • 作者单位

    Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics,The University of Tokyo, Tokyo 113-8656, Japan;

    Department of Applied Physics, The University of Tokyo, Tokyo 113-8656, Japan;

    Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics,The University of Tokyo, Tokyo 113-8656, Japan;

    Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics,The University of Tokyo, Tokyo 113-8656, Japan;

    Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Sendai 980-8577, Japan;

    Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics,The University of Tokyo, Tokyo 113-8656, Japan Department of Physics, The University of Tokyo, Tokyo 113-0033, Japan;

    Multiferroics Project, ERATO, Japan Science and Technology Agency (JST), c/o Department of Applied Physics,The University of Tokyo, Tokyo 113-8656, Japan Department of Applied Physics, The University of Tokyo, Tokyo 113-8656, Japan Cross-Correlated Material Research Group (CMRG), ASI, RIKEN, Wako, Saitama 351-0198, Japan;

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  • 正文语种 eng
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  • 关键词

    magnetomechanical and magnetoelectric effects, magnetostriction; ferromagnetic, antiferromagnetic, and ferrimagnetic resonances; spin-wave resonance; dynamic properties (dynamic susceptibility, spin waves, spin diffusion, dynamic scaling, etc.);

    机译:磁机械和磁电效应;磁致伸缩;铁磁;反铁磁和亚铁磁谐振;自旋波共振动态特性(动态磁化率;自旋波;自旋扩散;动态缩放等);

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