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Anomalous polarization of the photoluminescence from anisotropic colloidal CdSe nanocrystals subject to external magnetic fields

机译:各向异性胶体CdSe纳米晶体在外部磁场作用下的光致发光异常极化

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摘要

We explain anomalous polarization of magnetophotoluminescence from CdSe nanocrystals with built-in anisotropy observed by Htoon et ai, [Phys. Rev. Lett. 102, 017402 (2009)] in external magnetic fields up to 5 T. While there are two radiative doublets associated with the exciton ground state, it is the lower component of the upper doublet which demonstrates a truly anomalous behavior. We further describe complex behavior of the doublets components polarization in high-magnetic fields. The polarization degree of the upper component of each doublet varies with the applied magnetic field slower than that of the lower component. However, for the upper doublet this behavior is more pronounced and becomes apparent at much lower fields.
机译:我们解释了Htoon等人观察到的具有内置各向异性的CdSe纳米晶体的磁光致发光异常极化。牧师102,017402(2009)]在高达5 T的外部磁场中。尽管激子基态有两个辐射双峰态,但它是上部双峰态的下部分量,表现出真正的异常行为。我们进一步描述了在高磁场中双峰态分量极化的复杂行为。每个双峰的上半部分的极化度随施加的磁场的变化比下半部分的极化度慢。但是,对于上双峰,此行为更为明显,并且在低得多的场上变得明显。

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