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首页> 外文期刊>Physical review >Giant Rabi splitting between localized mixed plasmon-exciton states in a two-dimensional array of nanosize metallic disks in an organic semiconductor
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Giant Rabi splitting between localized mixed plasmon-exciton states in a two-dimensional array of nanosize metallic disks in an organic semiconductor

机译:在有机半导体中的纳米尺寸金属盘二维阵列中的局部混合等离子体激子状态之间的巨型拉比分裂

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摘要

We study localized surface plasmons in strong coupling with excitons of organic semiconductors. The plasmons are localized in lithographed silver nanodisks organized in square array. A giant Rabi splitting energy of 450 meV is obtained, and typical behaviors of mixed states, i.e., anticrossing of their energies and crossing of their linewidths, are observed. Three-dimensional finite-difference time-domain simulations and coupled oscillator calculations are used to analyze and corroborate the experimental results.
机译:我们研究与有机半导体的激子强耦合的局部表面等离子体激元。等离子体激元位于以正方形阵列组织的光刻银纳米盘中。获得了450meV的巨大拉比分裂能,并且观察到混合态的典型行为,即,它们的能量的反交叉和其线宽的交叉。三维有限差分时域仿真和耦合的振荡器计算被用来分析和证实实验结果。

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  • 来源
    《Physical review》 |2009年第3期|033303.1-033303.4|共4页
  • 作者单位

    Universite de Lyon Universite Lyon 1, LPMCN CNRS, UMR 5586, 69622 Villeurbanne, France GES, Universite Montpellier II-CNRS, Case Courrier 074, F-34095 Montpellier Cedex 5, France;

    Universite de Lyon Universite Lyon 1, LPMCN CNRS, UMR 5586, 69622 Villeurbanne, France;

    GES, Universite Montpellier II-CNRS, Case Courrier 074, F-34095 Montpellier Cedex 5, France;

    LPN, CNRS, Route de Nozay, F-91460 Marcoussis, France;

    Universite de Lyon Universite Lyon 1, LMI CNRS, UMR 5615, 69622 Villeurbanne, France;

    GES, Universite Montpellier II-CNRS, Case Courrier 074, F-34095 Montpellier Cedex 5, France;

    Universite de Lyon Universite Lyon 1, LPMCN CNRS, UMR 5586, 69622 Villeurbanne, France;

    Universite de Lyon Universite Lyon 1, LPMCN CNRS, UMR 5586, 69622 Villeurbanne, France;

    GES, Universite Montpellier II-CNRS, Case Courrier 074, F-34095 Montpellier Cedex 5, France;

    LPN, CNRS, Route de Nozay, F-91460 Marcoussis, France;

    GES, Universite Montpellier II-CNRS, Case Courrier 074, F-34095 Montpellier Cedex 5, France;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    polymers; organic compounds; excitons and related phenomena; collective excitations (including excitons, polarons, plasmons and other charge-density excitations); nanocrystals and nanoparticles;

    机译:聚合物有机化合物;激子和相关现象;集体激发(包括激子;极化子;等离激元和其他电荷密度激发);纳米晶体和纳米颗粒;

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