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Controlling the interactions between polaritons and molecular vibrations in strongly coupled organic semiconductor microcavities

机译:控制强耦合有机半导体微腔中极化子与分子振动之​​间的相互作用

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摘要

We study the microscopic processes that determine the dynamics of polaritons in strongly-coupled organic-semiconductor microcavities. Using a quantum kinetic theory, we show that resonant couplings and interactions between cavity photons, excitons, and localized molecular vibrations strongly affect the polariton resonance line shapes in J-aggregate microcavities. We use our many-body calculation to reproduce the measured polariton emission at exciton-photon resonance which is determined as a function of the Rabi-splitting energy.
机译:我们研究确定强耦合有机半导体微腔中极化子动力学的微观过程。使用量子动力学理论,我们表明腔光子,激子和局部分子振动之​​间的共振耦合和相互作用会强烈影响J聚​​集微腔中的极化子共振线形状。我们使用多体计算来重现在激子光子共振时测得的极化子发射,该极化子发射是拉比分裂能的函数。

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