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Magnetic Order In Ybmno_3 Studied By Neutron Diffraction And Moessbauer Spectroscopy

机译:中子衍射和莫斯鲍尔谱研究Ybmno_3的磁阶

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The magnetic ordering of the hexagonal multiferroic compound YbMnO_3 has been studied between 100 and 1.5 K by combining neutron powder diffraction, ~(170)Yb Mossbauer spectroscopy, and magnetization measurements. The Yb moments of the two crystallographic sites order at two different temperatures: the 4b site together with the Mn moments (at T_Napprox=85 K) and the 2α site well below (at 3.5 K). The temperature dependences of the Mn and Yb moments are explained within a molecular-field model, showing that the 4b and 2α sites order via Yb-Mn and Yb-Yb interactions, respectively. A simple picture taking into account the local Mn environment of the rare-earth R (4b) ion is proposed to couple R and Mn orders in hexagonal RMnO_3 manganites. The nature and symmetry of the R-Mn interactions yielding the R order are discussed.
机译:通过结合中子粉末衍射,〜(170)Yb Mossbauer光谱学和磁化强度测量,研究了六角形多铁化合物YbMnO_3的磁序在100和1.5 K之间。两个晶体学位点的Yb矩在两个不同的温度下有序:4b位点和Mn矩(在T_Napprox = 85 K时)和2α位在下面(在3.5 K时)。在分子场模型中解释了Mn和Yb矩的温度依赖性,表明4b和2α位分别通过Yb-Mn和Yb-Yb相互作用有序。提出了一个简单的图片,考虑了稀土R(4b)离子的局部Mn环境,以将R和Mn阶偶合在六方RMnO_3锰矿中。讨论了产生R阶的R-Mn相互作用的性质和对称性。

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