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Mimicking chiral light-matter interaction

机译:模仿手性光与物质的相互作用

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摘要

We demonstrate that achiral electric-dipole scatterers can mimic an interaction of light with chiral matter by generating far-field circular polarization upon scattering, even though the optical chirality of the incident field as well as that of the scattered light is zero. On the one hand, the presented effect originates from the fact that electric-dipole scatterers respond selectively only to the incident electric field, which eventually results in depolarization of the transmitted beam and in generation of far-field circular polarization. On the other hand, although the incident beam does not possess any optical chirality, it lacks reflection symmetry and therefore it is geometrically chiral. To experimentally demonstrate this effect, we utilize a cylindrical vector beam with spiral polarization and a spherical gold nanoparticle positioned on the optical axis-the axis of rotational symmetry of the system. Our experiment and a simple theoretical model address the fundamentals of duality symmetry in optics and chiral light-matter interactions, accentuating their richness and ubiquity yet in highly symmetric configurations.
机译:我们证明,即使入射场和散射光的光学手性为零,非手性电偶极散射体也可以通过在散射时产生远场圆偏振来模拟光与手性物质的相互作用。一方面,所呈现的效果源自以下事实:电偶极子散射仅选择性地对入射电场做出响应,这最终导致透射光束消偏振,并产生远场圆偏振。另一方面,尽管入射光束不具有任何光学手性,但它缺乏反射对称性,因此在几何上是手性的。为了通过实验证明这种效果,我们利用了具有螺旋偏振的圆柱形矢量束和位于光轴(系统的旋转对称轴)上的球形金纳米粒子。我们的实验和一个简单的理论模型解决了光学中的对偶对称性和手性光-质相互作用的基础,强调了它们的丰富性和普遍性,但仍具有高度对称的配置。

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  • 来源
    《Physical review》 |2019年第24期|241101.1-241101.6|共6页
  • 作者

    Nechayev Sergey; Banzer Peter;

  • 作者单位

    Max Planck Inst Sci Light, Staudtstr 2, D-91058 Erlangen, Germany;

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  • 原文格式 PDF
  • 正文语种 eng
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