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Optical study on the possible Slater insulator SrIr_(0.8)Sn_(0.2)O_3

机译:对可能的壁板绝缘体SRIR_(0.8)SN_(0.2)O_3的光学研究

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摘要

The orthorhombic perovskite iridate SrIr0.8Sn0.2O3 is reported to be a new candidate of Slater insulator at low temperatures. Here, we present optical spectroscopy measurements on SrIr0.8Sn0.2O3 at different temperatures (T) across the paramagnetic-antiferromagnetic phase transition. The low energy reflectivity decreases with reducing T . Six phonon peaks in the spectrum at low T are visible at room temperature, indicating the absence of crystal structure phase transition from 300 K to 10 K. The real part of conductivity spectra sigma(1)(omega) are obtained by employing the standard Kramers-Kronig transformation. In the paramagnetic state at room temperature, sigma(1)(omega) reaches a limiting value as omega - 0, implying an electrical conducting state. Upon decreasing T, the low frequency sigma(1)(omega) decreases and approaches zero with a concomitant opening of a direct gap. Detailed analysis of the low energy data shows that the gap opening is continuous and sigma(1)(omega) at the low energy gap edge follows an unusual omega(1/2). dependence at low temperatures which is remarkably similar to other Slater insulators, such as NaOsO3.
机译:据报道,正晶钙钙钛矿抗SRIR0.8SN0.2O3是低温下的莱特拉特绝缘体的新候选者。这里,我们在顺磁 - 反铁磁相转变的不同温度(t)上呈现SRIR0.8SN0.2O3上的光学光谱测量。低能量反射率降低了减少T.在室温下,低T的光谱中的六个声子峰可见,表示不存在从300k至10k的晶体结构相转变。通过使用标准克拉姆获得电导率光谱σ(1)(Omega)的实部-Kronig转换。在室温下的顺磁状态下,Sigma(1)(OMEGA)达到极限值,例如ω-> 0,暗示导电状态。在降低T时,低频Sigma(1)(OMEGA)降低并通过伴随的直接间隙的开口来降低零。低能量数据的详细分析表明,间隙开度是连续的,并且在低能量间隙边缘处的σ(1)(Omega)遵循不寻常的ω(1/2)。依赖于低温,这与其他类似的壁图绝缘体(例如Naoso3)相似。

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  • 来源
    《Physical review》 |2019年第4期|045101.1-045101.6|共6页
  • 作者单位

    Chinese Acad Sci Inst Phys Beijing Natl Lab Condensed Matter Phys Beijing 100190 Peoples R China;

    Chinese Acad Sci Inst Phys Beijing Natl Lab Condensed Matter Phys Beijing 100190 Peoples R China|Univ Chinese Acad Sci Sch Phys Sci Beijing 100190 Peoples R China;

    Chinese Acad Sci Inst Phys Beijing Natl Lab Condensed Matter Phys Beijing 100190 Peoples R China;

    Chinese Acad Sci Inst Phys Beijing Natl Lab Condensed Matter Phys Beijing 100190 Peoples R China|Univ Chinese Acad Sci Sch Phys Sci Beijing 100190 Peoples R China|Songshan Lake Mat Lab Dongguan 523808 Guangdong Peoples R China;

    Chinese Acad Sci Inst Phys Beijing Natl Lab Condensed Matter Phys Beijing 100190 Peoples R China|ShanghaiTech Univ Sch Phys Sci & Technol Shanghai 201210 Peoples R China;

    Boston Coll Dept Phys Chestnut Hill MA 02467 USA;

    Chinese Acad Sci Inst Phys Beijing Natl Lab Condensed Matter Phys Beijing 100190 Peoples R China|Univ Chinese Acad Sci Sch Phys Sci Beijing 100190 Peoples R China|Songshan Lake Mat Lab Dongguan 523808 Guangdong Peoples R China;

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