Modeling of Nickel Surface State in Electrocatalytic Hypophosphite Oxidation According to On-Line Electrochemical Mass Spectrometry Studies

Zenonas Jusys; Algirda Vaskelis

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Modeling of Nickel Surface State in Electrocatalytic Hypophosphite Oxidation According to On-Line Electrochemical Mass Spectrometry Studies

机译：在线电化学质谱研究电催化次磷酸盐氧化中镍表面态的建模

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Computer simulation of possible distribution of H_ad and D_ad atoms developed on nickel surface as a result of partial reactions of anodic hypophosphite oxidation and cathodic proton (deuteron) discharge from water respec- tively was used for modeling of the catalyst surface state according to on-line electrochemical mass spectrometry dta. The simplies lattice-gas model gives a probable qualitative description of the catalyst surface state and allows the genesis of electrocatalytic properties of nickel with the electrode potential to be followed.

机译：阳极次磷酸盐氧化和阴极质子（氘）从水中放电的部分反应的结果，计算机模拟了镍表面上H_ad和D_ad原子的可能分布，根据在线方法对催化剂的表面状态进行了建模。电化学质谱法简单的晶格气体模型给出了催化剂表面状态的可能的定性描述，并允许遵循电极电位的镍电催化性质的产生。

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《Berichte der Bunsengesellschaft fur Physikalische Chemie》 |1997年第12期|p.1865-1869|共5页
作者
Zenonas Jusys; Algirda Vaskelis;
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原文格式 PDF
正文语种 eng
中图分类化学;
关键词
Computer Simulation; Hypophosphite; Nickel; Isotopes;

机译：计算机仿真;次磷酸盐镍;同位素;

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5. A mass spectrometry study of the surface chemical activities of thorium oxide and cerium-doped thorium oxide. [D] . Grabbe, Alexis. 1989

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机译：电化学质谱。

Modeling of Nickel Surface State in Electrocatalytic Hypophosphite Oxidation According to On-Line Electrochemical Mass Spectrometry Studies

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