Tailoring Surface Electronic Properties to Promote Chemical Reactivity

E. Bertel; P. Sandl; K.D. Rendulic; M. Beutl

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Tailoring Surface Electronic Properties to Promote Chemical Reactivity

机译：调整表面电子特性以促进化学反应

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摘要

One of the foremost objectives in the search for improved catalysts is the promotion of molecule dissociation, which in many catalytic reactions is the rate limiting step. It is shown that modification of electronic surface states by surface dopants allows to control the dissociation barrier. The relation of this new type of promotion mechanism to the effect of surfactants in metal epitaxy opens a new perspective in the search for both, promoters and surfactants.

机译：寻找改进的催化剂的首要目的之一是促进分子解离，这在许多催化反应中是限速步骤。结果表明，通过表面掺杂剂对电子表面态的修饰可以控制解离势垒。这种新型的促进机制与表面活性剂在金属外延中的作用之间的关系为寻找促进剂和表面活性剂开辟了新的前景。

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来源
《Berichte der Bunsengesellschaft fur Physikalische Chemie》 |1996年第2期|p.114-118|共5页
作者
E. Bertel; P. Sandl; K.D. Rendulic; M. Beutl;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
关键词
catalysis; epitaxy; spectroscopy; photoelectron; surfaces;

机译：催化;外延;光谱学;光电子;表面;

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机译：弯曲应变定制磁性和电子传输性能反应溅射的γ'-Fe4N / Muscovite外延异质结构朝着柔性闪蒸
3. Tailoring Surface Properties through in Situ Functionality Gradients in Reactively Modified Poly(2-vinyl-4,4-dimethyl azlactone) Thin Films [J] . Bethany Aden, Dayton P. Street, Benjamin W. Hopkins, Langmuir: The ACS Journal of Surfaces and Colloids . 2018,第18期

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4. Chemicals from bioethanol: tailoring copper electronic properties to enhance its performance on the one-pot ethyl acetate synthesis [C] . Isabel C. De Freitas, Jean Marcel R. Gallo, Jose Maria C. Bueno AIChE Annual Meeting . 2014

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5. ELECTRONIC STRUCTURE AND REACTIVITY OF CHEMICALLY MODIFIED MOLYBDENUM(100) SURFACES AND APPLICATION OF PULSED LASER HEATING TO STUDIES OF SURFACE CHEMICAL PHENOMENA. [D] . GRANT, JOHN LEONARD. 1987

机译：化学修饰的钼（100）表面的电子结构和反应性以及脉冲激光加热在表面化学现象研究中的应用。
6. Observation and manipulation of subsurface hydride in Pd{111} and its effect on surface chemical physical and electronic properties [O] . E. Charles H. Sykes, Luis C. Fernández-Torres, Sanjini U. Nanayakkara, 2005

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7. Bending Strain Tailored Magnetic and Electronic Transport Properties of Reactively Sputtered -Fe4N/Muscovite Epitaxial Heterostructures toward Flexible Spintronics [O] . -1

机译：弯曲应变为反应溅射的磁力和电子传输性能，反应溅射-Fe4N / Muscovite外延异质结构朝着柔性闪光
8. How Much do Multiple Electronic Surfaces Influence Chemical Reactivity. F + HH: A Case Study. [R] . Komornicki, A., George, T. F., Morokuma, K. 1976

机译：多个电子表面对化学反应性有多大影响。 F + HH：案例研究。

Tailoring Surface Electronic Properties to Promote Chemical Reactivity

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