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首页> 外文期刊>Sensors and Actuators >In-situ one-step method for fabricating three-dimensional grass-like carbon-doped ZrO_2 films for room temperature alcohol and acetone sensors
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In-situ one-step method for fabricating three-dimensional grass-like carbon-doped ZrO_2 films for room temperature alcohol and acetone sensors

机译:一种用于室温酒精和丙酮传感器的三维草状碳掺杂ZrO_2薄膜的原位制备方法

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摘要

Carbon-doped ZrO_2 film with three-dimensional (3D) grass-like architecture was fabricated directly on interdigitated electrodes via one-step electrostatic spray deposition (ESD) using zirconatrane precursor without any additional carbon source and template. A one-step synthetic route was presented in which no additional film fabrication steps were required. The mesoporous micrograss structure comprised numerous interconnected nanoleaves. The synergistic combination of the unique morphology and carbon doping can offer superior room-temperature gas sensing activity for detecting alcohol and acetone. The sensitivity of the devices to methanol, ethanol, n-propanol and acetone was also tested. The gas sensing test results showed that the 3D hierarchical carbon-doped ZrO_2 based sensor exhibited excellent gas sensing performance at room temperature in terms of high response, short response/recovery times, good repeatability, long-term stability and superior selectivity to acetone, and has much higher response in comparison with the ZrO_2 sensor derived from commercial starting material.
机译:使用氧化锆前驱体通过一步静电喷涂(ESD)直接在叉指电极上制备了具有三维(3D)草状结构的碳掺杂ZrO_2膜,而无需使用任何其他碳源和模板。提出了一种一步合成路线,其中不需要额外的薄膜制造步骤。中孔微草结构包含许多相互连接的纳米叶。独特的形态和碳掺杂的协同组合可以提供出色的室温气体传感活性,以检测酒精和丙酮。还测试了设备对甲醇,乙醇,正丙醇和丙酮的敏感性。气敏测试结果表明,基于3D分层碳掺杂ZrO_2的传感器在室温下表现出出色的气敏性能,具有高响应,短响应/恢复时间,良好的重复性,长期稳定性和对丙酮的优异选择性,以及与衍生自商业原材料的ZrO_2传感器相比,具有更高的响应速度。

著录项

  • 来源
    《Sensors and Actuators》 |2017年第4期|202-214|共13页
  • 作者单位

    Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, Thailand;

    Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, Thailand;

    Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, Thailand,High Performance and Smart Materials, Center of Excellence for Petrochemical and Materials Technology, Chulalongkorn University, Bangkok, Thailand;

    Department of Materials Science and Engineering, Faculty of Engineering and Industrial Technology, Silpakorn University, Nakhon Pathom, Thailand,High Performance and Smart Materials, Center of Excellence for Petrochemical and Materials Technology, Chulalongkorn University, Bangkok, Thailand;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Carbon; Electrostatic spray deposition; Gas sensor; ZrO_2;

    机译:碳;静电喷涂沉积;气体传感器ZrO_2;

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