• 主题
高级搜索  >
历史搜索 清空历史
首页> 外文期刊>Theoretical and applied climatology >Assessment of the first indirect radiative effect of ammonium-sulfate-nitrate aerosols in East Asia
【24h】

Assessment of the first indirect radiative effect of ammonium-sulfate-nitrate aerosols in East Asia

机译：评估东亚硫酸铵-硝酸盐气溶胶的首次间接辐射效应

获取原文
获取原文并翻译 | 示例
           
页面导航
  • 摘要
  • 著录项
  • 相似文献
  • 相关主题

摘要

A physically based cloud nucleation parameterization was introduced into an optical properties/radiative transfer module incorporated with the off-line air quality modeling system Regional Atmospheric Modeling System (RAMS)-Models-3 Community Multi Scale Air Quality (CMAQ) to investigate the distribution features of the first indirect radiative effects of sulfate, nitrate, and ammonium-sulfate-nitrate (ASN) over East Asia for the years of 2005, 2010, and 2013. The relationship between aerosol particles and cloud droplet number concentration could be properly described by this parameterization because the simulated cloud fraction and cloud liquid water path were generally reliable compared with Moderate Resolution Imaging Spectroradiometer (MODIS) retrieved data. Simulation results showed that the strong effect of indirect forcing was mainly concentrated in Southeast China, the East China Sea, the Yellow Sea, and the Sea of Japan. The highest indirect radiative forcing of ASN reached -3.47 W m(-2) over Southeast China and was obviously larger than the global mean of the indirect forcing of all anthropogenic aerosols. In addition, sulfate provided about half of the contribution to the ASN indirect forcing effect. However, the effect caused by nitrate was weak because the mass burden of nitrate was very low during summer, whereas the cloud fraction was the highest. The analysis indicated that even though the interannual variation of indirect forcing magnitude generally followed the trend of aerosol mass burden from 2005 to 2013, the cloud fraction was an important factor that determined the distribution pattern of indirect forcing. The heaviest aerosol loading in North China did not cause a strong radiative effect because of the low cloud fraction over this region.
机译：将基于物理的云成核参数化引入光学特性/辐射传输模块，该模块与离线空气质量建模系统结合起来区域大气建模系统（RAMS）-Models-3社区多尺度空气质量（CMAQ）以研究分布特征硫酸盐，硝酸盐和硫酸铵-硝酸盐（ASN）在2005年，2010年和2013年对东亚的首次间接辐射效应。可以用此方法正确描述气溶胶颗粒与云滴数量浓度之间的关系。进行参数化是因为与中分辨率成像光谱仪（MODIS）检索到的数据相比，模拟的云量和云水路径通常是可靠的。仿真结果表明，间接强迫的强力效应主要集中在中国东南部，东海，黄海和日本海。在中国东南部，ASN的最高间接辐射强迫达到了-3.47 W m（-2），显然大于所有人为气溶胶间接强迫的全球平均值。此外，硫酸盐对ASN间接强迫作用的贡献约占一半。但是，由于夏季硝酸盐的质量负担非常低，而云雾含量最高，因此硝酸盐的影响很弱。分析表明，尽管间接强迫幅度的年际变化总体上遵循2005年至2013年气溶胶质量负担的趋势，但云量是决定间接强迫分布模式的重要因素。华北地区最重的气溶胶装载量并未引起强烈的辐射效应，因为该地区的云量较低。

著录项

  • 来源
    《Theoretical and applied climatology》 |2017年第4期|817-830|共14页
  • 作者

    Han Xiao; Zhang Meigen; Skorokhod Andrei;

  • 作者单位

    Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China;

    Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China|Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Urban Atmospher Environm, Xiamen 361021, Peoples R China;

    Russian Acad Sci, AM Obukhov Inst Atmospher Phys, Lab Atmospher Gas Species, Moscow 119017, Russia;

  • 收录信息
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

相似文献

  • 外文文献
  • 中文文献
  • 专利
获取原文

客服邮箱：kefu@zhangqiaokeyan.com

京公网安备：11010802029741号 ICP备案号：京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有

  • 客服微信

  • 服务号