Angular Distributions of Products in the Photodissociation of Diatomic Molecules

James L. Kinsey; Bruce R. Johnson

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Angular Distributions of Products in the Photodissociation of Diatomic Molecules

机译：双原子分子光解中产物的角分布

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The issue of angular distributions of the products of photodissociation of diatomic molecules is reexamined on two aspects: (1) the nature of the state that is prepared by excitation from a bound level into a continuum, and (2) a demonstration that a semiclassical connection between the J-derivative of the scattering phase shift and the classical deflection function leads to a recovery of the classical expression for correction of the angular distribution owing to finite rotation of the molecule during photodissociation. Higher-order quantum contributions to this correction also result from these observations.

机译：从两个方面重新审查了双原子分子光解离产物的角分布问题：（1）通过从束缚能级激发到连续体而制备的状态的性质，（2）证明了半经典连接由于光解离过程中分子的有限旋转，散射相移的J导数和经典偏转函数之间的差导致经典表达式的恢复，以校正角度分布。这些观察结果也为该校正提供了更高阶的量子贡献。

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《The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory》 |1998年第47期|共6页
作者
James L. Kinsey; Bruce R. Johnson;
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正文语种 eng
中图分类物理化学（理论化学）、化学物理学;
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1. Angular Distributions of Products in the Photodissociation of Diatomic Molecules [J] . James L. Kinsey, Bruce R. Johnson The journal of physical chemistry, A. Molecules, spectroscopy, kinetics, environment, & general theory . 1998,第45a48期

机译：双原子分子光解中产物的角分布
2. Photofragment angular momentum distributions in the molecular frame. III. Coherent effects in the photodissociation of polyatomic molecules with circularly polarized light [J] . Rakitzis T.P. The Journal of Chemical Physics . 2010,第20期

机译：分子框架中的光碎角动量分布。三，多原子分子与圆偏振光光解离中的相干效应
3. Rotational and angular distributions of NO products from NO-Rg (Rg = He, Ne, Ar) complex photodissociation [J] . Holmes-Ross Heather L., Valenti Rebecca J., Yu Hua-Gen, The Journal of Chemical Physics . 2016,第4期

机译：NO-Rg（Rg = He，Ne，Ar）复杂光解过程中NO产物的旋转和角度分布
4. Vibrationally resolved molecular frame photoelectron angular distributions of diatomic and polyatomic molecules [C] . Etienne Plésiat, Piero Decleva, Fernando Martin ICPEAC . 2014

机译：振动解析的分子框架光电子硅藻和多原子分子的角度分布
5. Photoelectron angular and energy distributions from the resonant two-photon ionization of diatomic sodium. [D] . DANIEL, ROBERT GEORGE. 1991

机译：双原子钠共振双光子电离的光电子角和能量分布。
6. Photodissociation of ClNO in the 2 1A′ State: Computational and Experimental NO Product State Distributions [O] . Kiera M Jones, Jadwiga A Milkiewicz, Benjamin J Whitaker, -1

机译：ClNO在2 1A状态下的光解离：计算和实验的NO产物状态分布
7. Photofragment angular momentum distributions in the molecular frame. II. Single state dissociation, multiple state interference, and nonaxial recoil in photodissociation of polyatomic molecules [O] . Rakitzis, T. P., Alexander, A. J. 2010

机译：分子框架中的光碎片角动量分布。 II。单原子解离，多态干涉和多原子分子光解离中的非轴向反冲

Angular Distributions of Products in the Photodissociation of Diatomic Molecules

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