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Friction of Ionic Liquid–Glycol Ether Mixtures at Titanium Interfaces: Negative Load Dependence

机译：钛接口的离子液 - 乙二醇醚混合物的摩擦：负载依赖性

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Abstract >The atomic force microscopy experiments and nonequilibrium molecular dynamics (NEMD) simulations demonstrate a negative friction–load dependence to ionic liquid–glycol ether mixtures, that is, the friction decreases as the normal load increases. NEMD simulations reveal a structural reorientation of the studied ionic liquid (IL): as the normal load increases, the cation alkyl chains of ILs change the orientation to preferentially parallel to the tip scanning path. The flat‐oriented IL structures, similar to the “blooming lotus leaf,” produce a new sliding interface and reduce the friction. A further molecular dynamics simulation is carried out by adopting slit‐pore models to mimic the tip approaching process to confirm the dynamics of ILs. A faster diffusion of ILs in the smaller slit pore is observed. The faster diffusion of ILs in the more confined slit pore facilitates the structural reorientation of ILs. The resulted new sliding surface is responsible for the observed smaller friction at higher loads, also known as the negative friction–load dependence. These findings provide a fundamental explanation to the role of ILs in interfacial lubrications. They help to understand liquid flow properties under confinement, with implications for the development of better nanofluidic devices. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >原子力显微镜实验和非分子动力学（NEMD）模拟证明了对离子液 - 乙二醇醚混合物的负摩擦负荷依赖性，即，随着正常负载的增加，摩擦降低。 NEMD模拟揭示了所研究的离子液体（IL）的结构重新定位：随着正常负荷增加，ILS的阳离子烷基链改变为优先平行于尖端扫描路径的方向。面向扁平的IL结构，类似于“盛开的莲花”，产生新的滑动界面并减少摩擦。通过采用狭缝孔模型来实现进一步的分子动力学模拟以模拟尖端接近过程以确认ILS的动态。观察到ILS在较小的狭缝孔中的更快扩散。 ILS在更狭窄的狭缝孔中的速度扩散促进了ILS的结构重新定位。得到的新滑动表面负责在较高载荷下观察到的较小摩擦，也称为负摩擦负载依赖性。这些发现对ILS在界面润滑中的作用提供了根本的解释。他们有助于了解限制的液体流动性能，对更好的纳米流体装置的开发有影响。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第14期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=An Rong&option=202" target="_blank" rel="nofollow">An Rong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhou Guobing&option=202" target="_blank" rel="nofollow">Zhou Guobing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Yudan&option=202" target="_blank" rel="nofollow">Zhu Yudan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Wei&option=202" target="_blank" rel="nofollow">Zhu Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Liangliang&option=202" target="_blank" rel="nofollow">Huang Liangliang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shah Faiz Ullah&option=202" target="_blank" rel="nofollow">Shah Faiz Ullah;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Herbert Gleiter Institute of NanoscienceNanjing University of Science and TechnologyNanjing 210094 P. R. China;</p> <p>School of ChemicalUniversity of OklahomaNorman OK 73019 USA;</p> <p>State Key Laboratory of Materials‐Oriented Chemical EngineeringNanjing Tech UniversityNanjing 210009 P. R. China;</p> <p>State Key Laboratory of Materials‐Oriented Chemical EngineeringNanjing Tech UniversityNanjing 210009 P. R. China;</p> <p>School of ChemicalUniversity of OklahomaNorman OK 73019 USA;</p> <p>Chemistry of InterfacesLule? University of TechnologyS‐97187 Lule? Sweden;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=atomic force microscopy&option=203" rel="nofollow">atomic force microscopy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=friction&option=203" rel="nofollow">friction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ionic liquid&option=203" rel="nofollow">ionic liquid;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=negative&option=203" rel="nofollow">negative;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=structural change&option=203" rel="nofollow">structural change;</a> </p> <div class="translation"> 机译：原子力显微镜;摩擦;离子液体;负;结构变化; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022435728.html">Friction: Friction of Ionic Liquid–Glycol Ether Mixtures at Titanium Interfaces: Negative Load Dependence (Adv. 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=田征&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 田征</a> <span> . 2013</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061201547856.html">利用离子液体/聚苯胺制备的多孔碳负载二氧化钛复合材料及其方法和应用</a> <b>[P]</b> . <span> 中国专利： CN103349971B </span> <span> . 2015.02.04</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120101970270.html">利用离子液体/聚苯胺制备的多孔碳负载二氧化钛复合材料及其方法和应用</a> <b>[P]</b> . <span> 中国专利： CN103349971A </span> <span> . 2013-10-16</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130401878683.html">Application of ionic liquid in propylene glycol ether synthesis and method for synthesizing propylene glycol ether</a> <b>[P]</b> . <span> 外国专利： <!-- 美国专利： --> US10604468B2 </span> <span> . 2020-03-31</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：离子液体在丙二醇醚合成中的应用及丙二醇醚的合成方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130406883187.html">APPLICATION OF IONIC LIQUID IN PROPYLENE GLYCOL ETHER SYNTHESIS AND METHOD FOR SYNTHESIZING PROPYLENE GLYCOL ETHER</a> <b>[P]</b> . <span> 外国专利： <!-- 美国专利： --> US2018222833A1 </span> <span> . 2018-08-09</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：离子液体在丙二醇醚合成中的应用及丙二醇醚的合成方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130406396373.html">APPLICATION OF IONIC LIQUID IN PROPYLENE GLYCOL ETHER SYNTHESIS AND METHOD FOR SYNTHESIZING PROPYLENE GLYCOL ETHER</a> <b>[P]</b> . <span> 外国专利： <!-- 世界知识产权组织专利： --> WO2017197857A1 </span> <span> . 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